Your browser doesn't support javascript.
loading
Mostrar: 20 | 50 | 100
Resultados 1 - 20 de 18.914
Filtrar
1.
J Environ Sci (China) ; 149: 126-138, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181628

RESUMEN

With the continuous control of anthropogenic emissions, China's air quality has improved significantly in recent years. Given this background, research on how the short-term exposure risks caused by air pollution in China have changed is insufficient. This study utilized hourly concentration data from ground observation stations and the official air quality guidelines of the Ministry of Ecology and Environment of China and the World Health Organization as standards to systematically investigate the spatiotemporal characteristics and short-term exposure risks of air pollution in China from 2015 to 2022. The results indicate that various atmospheric pollutants except for ozone showed a decreasing trend yearly. Nationwide, both single pollutant air pollution days (SAPDs) and multiple pollutant air pollution days (MAPDs) showed varying degrees of reduction within 15 and 25 days, respectively. SAPD was dominated mainly by excessive PM2.5 and PM10 pollutants, while MAPD was dominated mainly by excessive pollutant combinations, including PM2.5 + PM10, CO + PM2.5 + PM10, and SO2 + PM2.5 + PM10. As the concentration of atmospheric pollutants decreased, the total excess risk (ER) decreased yearly from 2015 to 2022, but there were significant regional differences. Now, the ER is less than 0.25% in southern China, in the range of 0.25%-0.5% in the North China Plain and some cities in the northeast, and higher than 1% in the northwest. Particulate matter is currently the primary pollutant posing short-term exposure risk in China, especially due to the impact of sandstorm weather. This study indicates that China's atmospheric cleaning action is significantly beneficial for reducing health risks.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , Exposición a Riesgos Ambientales , Monitoreo del Ambiente , Material Particulado , China , Contaminación del Aire/estadística & datos numéricos , Contaminantes Atmosféricos/análisis , Material Particulado/análisis , Humanos , Medición de Riesgo
2.
J Environ Sci (China) ; 149: 200-208, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181634

RESUMEN

The acidity of atmospheric aerosols influences fundamental physicochemical processes that affect climate and human health. We recently developed a novel and facile water-probe-based method for directly measuring of the pH for micrometer-size droplets, providing a promising technique to better understand aerosol acidity in the atmosphere. The complex chemical composition of fine particles in the ambient air, however, poses certain challenges to using a water-probe for pH measurement, including interference from interactions between compositions and the influence of similar compositions on water structure. To explore the universality of our method, it was employed to measure the pH of ammonium, nitrate, carbonate, sulfate, and chloride particles. The pH of particles covering a broad range (0-14) were accurately determined, thereby demonstrating that our method can be generally applied, even to alkaline particles. Furthermore, a standard spectral library was developed by integrating the standard spectra of common hydrated ions extracted through the water-probe. The library can be employed to identify particle composition and overcome the spectral overlap problem resulting from similar effects. Using the spectral library, all ions were identified and their concentrations were determined, in turn allowing successful pH measurement of multicomponent (ammonium-sulfate-nitrate-chloride) particles. Insights into the synergistic effect of Cl-, NO3-, and NH4+ depletion obtained with our approach revealed the interplay between pH and volatile partitioning. Given the ubiquity of component partitioning and pH variation in particles, the water probe may provide a new perspective on the underlying mechanisms of aerosol aging and aerosol-cloud interaction.


Asunto(s)
Aerosoles , Monitoreo del Ambiente , Espectrometría Raman , Agua , Concentración de Iones de Hidrógeno , Espectrometría Raman/métodos , Agua/química , Monitoreo del Ambiente/métodos , Aerosoles/análisis , Contaminantes Atmosféricos/análisis , Contaminantes Atmosféricos/química , Atmósfera/química , Material Particulado/análisis
3.
J Environ Sci (China) ; 149: 342-357, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181647

RESUMEN

The toxicity of PM2.5 does not necessarily change synchronously with its mass concentration. In this study, the chemical composition (carbonaceous species, water-soluble ions, and metals) and oxidative potential (dithiothreitol assay, DTT) of PM2.5 were investigated in 2017/2018 and 2022 in Xiamen, China. The decrease rate of volume-normalized DTT (DTTv) (38%) was lower than that of PM2.5 (55%) between the two sampling periods. However, the mass-normalized DTT (DTTm) increased by 44%. Clear seasonal patterns with higher levels in winter were found for PM2.5, most chemical constituents and DTTv but not for DTTm. The large decrease in DTT activity (84%-92%) after the addition of EDTA suggested that water-soluble metals were the main contributors to DTT in Xiamen. The increased gap between the reconstructed and measured DTTv and the stronger correlations between the reconstructed/measured DTT ratio and carbonaceous species in 2022 were observed. The decrease rates of the hazard index (32.5%) and lifetime cancer risk (9.1%) differed from those of PM2.5 and DTTv due to their different main contributors. The PMF-MLR model showed that the contributions (nmol/(min·m3)) of vehicle emission, coal + biomass burning, ship emission and secondary aerosol to DTTv in 2022 decreased by 63.0%, 65.2%, 66.5%, and 22.2%, respectively, compared to those in 2017/2018, which was consistent with the emission reduction of vehicle exhaust and coal consumption, the adoption of low-sulfur fuel oil used on board ships and the reduced production of WSOC. However, the contributions of dust + sea salt and industrial emission increased.


Asunto(s)
Contaminantes Atmosféricos , Monitoreo del Ambiente , Material Particulado , Material Particulado/análisis , China , Contaminantes Atmosféricos/análisis , Oxidación-Reducción , Ciudades , Contaminación del Aire/estadística & datos numéricos
4.
J Environ Sci (China) ; 149: 431-443, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181655

RESUMEN

To investigate the seasonal characteristics in air pollution in Chengdu, a single particle aerosol mass spectrometry was used to continuously observe atmospheric fine particulate matter during one-month periods in summer and winter, respectively. The results showed that, apart from O3, the concentrations of other pollutants (CO, NO2, SO2, PM2.5 and PM10) were significantly higher in winter than in summer. All single particle aerosols were divided into seven categories: biomass burning (BB), coal combustion (CC), Dust, vehicle emission (VE), K mixed with nitrate (K-NO3), K mixed with sulfate and nitrate (K-SN), and K mixed with sulfate (K-SO4) particles. The highest contributions in both seasons were VE particles (24%). The higher contributions of K-SO4 (16%) and K-NO3 (10%) particles occurred in summer and winter, respectively, as a result of their different formation mechanisms. S-containing (K-SO4 and K-SN), VE, and BB particles caused the evolution of pollution in both seasons, and they can be considered as targets for future pollution reduction. The mixing of primary sources particles (VE, Dust, CC, and BB) with secondary components was stronger in winter than in summer. In summer, as pollution worsens, the mixing of primary sources particles with 62 [NO3]- weakened, but the mixing with 97 [HSO4]- increased. However, in winter, the mixing state of particles did not exhibit an obvious evolution rules. The potential source areas in summer were mainly distributed in the southern region of Sichuan, while in winter, besides the southern region, the contribution of the western region cannot be ignored.


Asunto(s)
Aerosoles , Contaminantes Atmosféricos , Contaminación del Aire , Monitoreo del Ambiente , Material Particulado , Estaciones del Año , Aerosoles/análisis , Contaminantes Atmosféricos/análisis , Material Particulado/análisis , China , Contaminación del Aire/estadística & datos numéricos , Espectrometría de Masas , Tamaño de la Partícula
5.
J Environ Sci (China) ; 149: 456-464, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181657

RESUMEN

Nitrogen-containing organic compounds (NOCs) may potentially contribute to aqueous secondary organic aerosols, yet the different formation of NOCs in aerosol particles and cloud droplets remains unclear. With the in-situ measurements performed at a mountain site (1690 m a.s.l.) in southern China, we investigated the formation of NOCs in the cloud droplets and the cloud-free particles, based on their mixing state information of NOCs-containing particles by single particle mass spectrometry. The relative abundance of NOCs in the cloud-free particles was significantly higher than those in cloud residual (cloud RES) particles. NOCs were highly correlated with carbonyl compounds (including glyoxalate and methylglyoxal) in the cloud-free particles, however, limited correlation was observed for cloud RES particles. Analysis of their mixing state and temporal variations highlights that NOCs was mainly formed from the carbonyl compounds and ammonium in the cloud-free particles, rather than in the cloud RES particles. The results support that the formation of NOCs from carbonyl compounds is facilitated in concentrated solutions in wet aerosols, rather than cloud droplets. In addition, we have identified the transport of biomass burning particles that facilitate the formation of NOCs, and that the observed NOCs is most likely contributed to the light absorption. These findings have implications for the evaluation of NOCs formation and their contribution to light absorption.


Asunto(s)
Aerosoles , Contaminantes Atmosféricos , Monitoreo del Ambiente , Nitrógeno , Compuestos Orgánicos , Aerosoles/análisis , Contaminantes Atmosféricos/análisis , Contaminantes Atmosféricos/química , Nitrógeno/química , Nitrógeno/análisis , Compuestos Orgánicos/química , China , Atmósfera/química , Material Particulado/análisis , Material Particulado/química
6.
J Environ Sci (China) ; 149: 57-67, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181668

RESUMEN

Size-fractionated particulate matter (PM2.5 and PM>2.5) was collected at a traffic site in Kanazawa, Japan in a seasonal sampling work in 2020. Nine polycyclic aromatic hydrocarbons (4- to 6-ring PAHs) were determined in fine and coarse particles. The gas/particle partitioning coefficients (Kp) of the PAHs were calculated from the supercooled liquid vapour pressure and octanol-air partitioning coefficient based on the relationships obtained in previous traffic pollution-related studies. Gaseous PAHs were estimated by Kp and the concentrations of PM and particulate PAHs. The concentrations of total PAHs were 32.5, 320.1 and 5646.2 pg/m3 in the PM>2.5, PM2.5 and gas phases, respectively. Significant seasonal trends in PAHs were observed (particle phase: lowest in summer, gas phase: lowest in spring, particle and gas phase: lowest in spring). Compared to 2019, the total PAH concentrations (in particles) decreased in 2020, especially in spring and summer, which might be due to reduced traffic trips during the COVID-19 outbreak. The incremental lifetime cancer risk (ILCR) calculated from the toxic equivalent concentrations relative to benzo[a]pyrene (BaPeq) was lower than the acceptable limit issued by the US Environmental Protection Agency, indicating a low cancer risk in long-term exposure to current PAH levels. It is notable that gaseous PAHs considerably contributed to BaPeq and ILCR (over 50%), which highlighted the significance of gaseous PAH monitoring for public health protection. This low-cost estimation method for gaseous PAHs can be expected to reliably and conveniently obtain PAH concentrations as a surrogate for traditional sampling in the future work.


Asunto(s)
Contaminantes Atmosféricos , Monitoreo del Ambiente , Material Particulado , Hidrocarburos Policíclicos Aromáticos , Hidrocarburos Policíclicos Aromáticos/análisis , Japón , Contaminantes Atmosféricos/análisis , Monitoreo del Ambiente/métodos , Material Particulado/análisis , Emisiones de Vehículos/análisis , Estaciones del Año
7.
J Environ Sci (China) ; 149: 564-573, 2025 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-39181667

RESUMEN

Airborne microorganisms (AM) have significant environmental and health implications. Extensive studies have been conducted to investigate the factors influencing the composition and diversity of AM. However, the knowledge of AM with anthropogenic activities has not reach a consensus. In this study, we took advantage of the dramatic decline of outdoor anthropogenic activities resulting from COVID-19 lockdown to reveal their associations. We collected airborne particulate matter before and during the lockdown period in two cities. The results showed that it was fungal diversity and communities but not bacteria obviously different between pre-lockdown and lockdown samples, suggesting that airborne fungi were more susceptible to anthropogenic activities than bacteria. However, after the implementation of lockdown, the co-occurrence networks of both bacterial and fungal community became more complex, which might be due to the variation of microbial sources. Furthermore, Mantel test and correlation analysis showed that air pollutants also partly contributed to microbial alterations. Airborne fungal community was more affected by air pollutants than bacterial community. Notably, some human pathogens like Nigrospora and Arthrinium were negatively correlated with air pollutants. Overall, our study highlighted the more impacts of anthropogenic activities on airborne fungal community than bacterial community and advanced the understanding of associations between anthropogenic activities and AM.


Asunto(s)
Microbiología del Aire , Contaminantes Atmosféricos , Bacterias , Monitoreo del Ambiente , Hongos , Bacterias/clasificación , Contaminantes Atmosféricos/análisis , Material Particulado/análisis , COVID-19 , Humanos , China
8.
J Environ Sci (China) ; 148: 409-419, 2025 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-39095176

RESUMEN

Sedimentation sludge water (SSW), a prominent constituent of wastewater from drinking water treatment plants, has received limited attention in terms of its treatment and utilization likely due to the perceived difficulties associated with managing SSW sludge. This study comprehensively evaluated the water quality of SSW by comparing it to a well-documented wastewater (filter backwash water (FBW)). Furthermore, it investigated the pollutant variations in the SSW during pre-sedimentation process, probed the underlying reaction mechanism, and explored the feasibility of employing a pilot-scale coagulation-sedimentation process for SSW treatment. The levels of most water quality parameters were generally comparable between SSW and FBW. During the pre-sedimentation of SSW, significant removal of turbidity, bacterial counts, and dissolved organic matter (DOM) was observed. The characterization of DOM components, molecular weight distributions, and optical properties revealed that the macromolecular proteinaceous biopolymers and humic acids were preferentially removed. The characterization of particulates indicated that high surface energy, zeta potential, and bridging/adsorption/sedimentation/coagulation capacities in aluminum residuals of SSW, underscoring its potential as a coagulant and promoting the generation and sedimentation of inorganic-organic complexes. The coagulation-sedimentation process could effectively remove pollutants from low-turbidity SSW ([turbidity]0 < 15 NTU). These findings provide valuable insights into the water quality dynamics of SSW during the pre-sedimentation process, facilitating the development of SSW quality management and enhancing its reuse rate.


Asunto(s)
Aguas del Alcantarillado , Eliminación de Residuos Líquidos , Eliminación de Residuos Líquidos/métodos , Aguas del Alcantarillado/química , Material Particulado/análisis , Aguas Residuales/química , Contaminantes Químicos del Agua/análisis , Purificación del Agua/métodos , Sustancias Húmicas/análisis , Calidad del Agua
9.
J Environ Sci (China) ; 148: 46-56, 2025 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-39095180

RESUMEN

Thermodynamic modeling is still the most widely used method to characterize aerosol acidity, a critical physicochemical property of atmospheric aerosols. However, it remains unclear whether gas-aerosol partitioning should be incorporated when thermodynamic models are employed to estimate the acidity of coarse particles. In this work, field measurements were conducted at a coastal city in northern China across three seasons, and covered wide ranges of temperature, relative humidity and NH3 concentrations. We examined the performance of different modes of ISORROPIA-II (a widely used aerosol thermodynamic model) in estimating aerosol acidity of coarse and fine particles. The M0 mode, which incorporates gas-phase data and runs the model in the forward mode, provided reasonable estimation of aerosol acidity for coarse and fine particles. Compared to M0, the M1 mode, which runs the model in the forward mode but does not include gas-phase data, may capture the general trend of aerosol acidity but underestimates pH for both coarse and fine particles; M2, which runs the model in the reverse mode, results in large errors in estimated aerosol pH for both coarse and fine particles and should not be used for aerosol acidity calculations. However, M1 significantly underestimates liquid water contents for both fine and coarse particles, while M2 provides reliable estimation of liquid water contents. In summary, our work highlights the importance of incorporating gas-aerosol partitioning when estimating coarse particle acidity, and thus may help improve our understanding of acidity of coarse particles.


Asunto(s)
Aerosoles , Contaminantes Atmosféricos , Modelos Químicos , Termodinámica , Aerosoles/análisis , Aerosoles/química , Contaminantes Atmosféricos/química , Contaminantes Atmosféricos/análisis , China , Monitoreo del Ambiente/métodos , Material Particulado/química , Material Particulado/análisis , Concentración de Iones de Hidrógeno , Tamaño de la Partícula
10.
J Environ Sci (China) ; 148: 591-601, 2025 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-39095192

RESUMEN

To explore air contamination resulting from special biomass combustion and suspended dust in Lhasa, the present study focused on the size distribution and chemical characteristics of particulate matter (PM) emission resulting from 7 types of non-fossil pollution sources. We investigated the concentration and size distribution of trace elements from 7 pollution sources collected in Lhasa. Combining Lhasa's atmospheric particulate matter data, enrichment factors (EFs) have been calculated to examine the potential impact of those pollution sources on the atmosphere quality of Lhasa. The highest mass concentration of total elements of biomass combustion appeared at PM0.4, and the second highest concentration existed in the size fraction 0.4-1 µm; the higher proportion (12 %) of toxic metals was produced by biomass combustion. The elemental composition of suspended dust and atmospheric particulate matter was close (except for As and Cd); the highest concentration of elements was all noted in PM2.5-10 (PM3-10). Potassium was found to be one of the main biomass markers. The proportion of Cu in suspended dust is significantly lower than that of atmospheric particulate matter (0.53 % and 3.75 %), which indicates that there are other anthropogenic sources. The EFs analysis showed that the Cr, Cu, Zn, and Pb produced by biomass combustion were highly enriched (EFs > 100) in all particle sizes. The EFs of most trace elements increased with decreasing particle size, indicating the greater influence of humanfactors on smaller particles.


Asunto(s)
Aerosoles , Contaminantes Atmosféricos , Polvo , Monitoreo del Ambiente , Tamaño de la Partícula , Material Particulado , Contaminantes Atmosféricos/análisis , Aerosoles/análisis , Material Particulado/análisis , Polvo/análisis , Oligoelementos/análisis , Contaminación del Aire/estadística & datos numéricos , Contaminación del Aire/análisis , China , Atmósfera/química
11.
J Environ Sci (China) ; 148: 702-713, 2025 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-39095202

RESUMEN

Chinese diesel trucks are the main contributors to NOx and particulate matter (PM) vehicle emissions. An increase in diesel trucks could aggravate air pollution and damage human health. The Chinese government has recently implemented a series of emission control technologies and measures for air quality improvement. This paper summarizes recent control technologies and measures for diesel truck emissions in China and introduces the comprehensive application of control technologies and measures in Beijing-Tianjin-Hebei and surrounding regions. Remote online monitoring technology has been adopted according to the China VI standard for heavy-duty diesel trucks, and control measures such as transportation structure adjustment and heavy pollution enterprise classification control continue to support the battle action plan for pollution control. Perspectives and suggestions are provided for promoting pollution control and supervision of diesel truck emissions: adhere to the concept of overall management and control, vigorously promote the application of systematic and technological means in emission monitoring, continuously facilitate cargo transportation structure adjustment and promote new energy freight vehicles. This paper aims to accelerate the implementation of control technologies and measures throughout China. China is endeavouring to control diesel truck exhaust pollution. China is willing to cooperate with the world to protect the global ecological environment.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , Monitoreo del Ambiente , Material Particulado , Emisiones de Vehículos , Emisiones de Vehículos/análisis , China , Contaminantes Atmosféricos/análisis , Contaminación del Aire/prevención & control , Contaminación del Aire/estadística & datos numéricos , Monitoreo del Ambiente/métodos , Material Particulado/análisis , Vehículos a Motor
12.
Sci Rep ; 14(1): 20630, 2024 09 04.
Artículo en Inglés | MEDLINE | ID: mdl-39232024

RESUMEN

We implemented a crossover study design exposing 15 participants to two indoor air quality conditions in the Well Living Lab. The first condition, the Standard Control Condition, resembled the ventilation and air supply of a typical home in the USA with a manually operated stove hood. The second condition, Advanced Control, had an automated: (i) stove hood, (ii) two portable air cleaners (PAC), and (iii) bathroom exhaust. The PM2.5 sensors were placed in the kitchen, living room, bedroom, and bathroom. Once the sensor detected a PM2.5 level of 15 µg/m3 or higher, an air quality intervention (stove hood, PAC or bathroom exhaust) in that space was activated and turned off when the corresponding PM2.5 sensor had three consecutive readings below 6 µg/m3. Advanced Control in the overall apartment reduced PM2.5 concentration by 40% compared to the Standard Control. The PM2.5 concentration difference between Advanced and Standard Control was ~ 20% in the kitchen. This can be attributed to using the stove hood manually in 66.5% of cooking PM2.5 emission events for 323.6 h compared to 88 h stove hood used in automated mode alongside 61.9 h and 33.7 h of PAC use in living room and bedroom, respectively.


Asunto(s)
Contaminación del Aire Interior , Culinaria , Vivienda , Material Particulado , Ventilación , Contaminación del Aire Interior/análisis , Contaminación del Aire Interior/prevención & control , Culinaria/métodos , Culinaria/instrumentación , Humanos , Material Particulado/análisis , Ventilación/métodos , Estudios Cruzados , Automatización , Monitoreo del Ambiente/métodos , Contaminantes Atmosféricos/análisis
13.
Lancet Planet Health ; 8(9): e657-e665, 2024 Sep.
Artículo en Inglés | MEDLINE | ID: mdl-39243781

RESUMEN

BACKGROUND: Ambient air pollution, including particulate matter (such as PM10 and PM2·5) and nitrogen dioxide (NO2), has been linked to increases in mortality. Whether populations' vulnerability to these pollutants has changed over time is unclear, and studies on this topic do not include multicountry analysis. We evaluated whether changes in exposure to air pollutants were associated with changes in mortality effect estimates over time. METHODS: We extracted cause-specific mortality and air pollution data collected between 1995 and 2016 from the Multi-Country Multi-City (MCC) Collaborative Research Network database. We applied a two-stage approach to analyse the short-term effects of NO2, PM10, and PM2·5 on cause-specific mortality using city-specific time series regression analyses and multilevel random-effects meta-analysis. We assessed changes over time using a longitudinal meta-regression with time as a linear fixed term and explored potential sources of heterogeneity and two-pollutant models. FINDINGS: Over 21·6 million cardiovascular and 7·7 million respiratory deaths in 380 cities across 24 countries over the study period were included in the analysis. All three air pollutants showed decreasing concentrations over time. The pooled results suggested no significant temporal change in the effect estimates per unit exposure of PM10, PM2·5, or NO2 and mortality. However, the risk of cardiovascular mortality increased from 0·37% (95% CI -0·05 to 0·80) in 1998 to 0·85% (0·55 to 1·16) in 2012 with a 10 µg/m3 increase in PM2·5. Two-pollutant models generally showed similar results to single-pollutant models for PM fractions and indicated temporal differences for NO2. INTERPRETATION: Although air pollution levels decreased during the study period, the effect sizes per unit increase in air pollution concentration have not changed. This observation might be due to the composition, toxicity, and sources of air pollution, as well as other factors, such as socioeconomic determinants or changes in population distribution and susceptibility. FUNDING: None.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , Enfermedades Cardiovasculares , Ciudades , Dióxido de Nitrógeno , Material Particulado , Enfermedades Respiratorias , Contaminación del Aire/efectos adversos , Contaminación del Aire/análisis , Humanos , Material Particulado/análisis , Material Particulado/efectos adversos , Enfermedades Cardiovasculares/mortalidad , Dióxido de Nitrógeno/análisis , Dióxido de Nitrógeno/efectos adversos , Contaminantes Atmosféricos/efectos adversos , Contaminantes Atmosféricos/análisis , Enfermedades Respiratorias/mortalidad , Enfermedades Respiratorias/inducido químicamente , Exposición a Riesgos Ambientales/efectos adversos
14.
Proc Natl Acad Sci U S A ; 121(38): e2401882121, 2024 Sep 17.
Artículo en Inglés | MEDLINE | ID: mdl-39250663

RESUMEN

Although it is well documented that exposure to fine particulate matter (PM2.5) increases the risk of several adverse health outcomes, less is known about its relationship with economic opportunity. Previous studies have relied on regression modeling, which implied strict assumptions regarding confounding adjustments and did not explore geographical heterogeneity. We obtained data for 63,165 US census tracts (86% of all census tracts in the United States) on absolute upward mobility (AUM) defined as the mean income rank in adulthood of children born to families in the 25th percentile of the national income distribution. We applied and compared several state-of-the-art confounding adjustment methods to estimate the overall and county-specific associations of childhood exposure to PM2.5 and AUM controlling for many census tract-level confounders. We estimate that census tracts with a 1 µg/m3 higher PM2.5 concentrations in 1982 are associated with a statistically significant 1.146% (95% CI: 0.834, 1.458) lower AUM in 2015, on average. We also showed evidence that this relationship varies spatially between counties, exhibiting a more pronounced negative relationship in the Midwest and the South.


Asunto(s)
Exposición a Riesgos Ambientales , Material Particulado , Material Particulado/análisis , Estados Unidos , Humanos , Exposición a Riesgos Ambientales/efectos adversos , Niño , Contaminantes Atmosféricos/análisis , Renta , Contaminación del Aire/análisis , Contaminación del Aire/efectos adversos , Femenino
15.
Ying Yong Sheng Tai Xue Bao ; 35(7): 2013-2024, 2024 Jul 18.
Artículo en Inglés | MEDLINE | ID: mdl-39233432

RESUMEN

Plants could effectively adsorb and remove particulate matter from the air, while could be suffered from the adverse effects. Therefore, exploring the interaction between plants and atmospheric particulate matter is crucial for profound understanding of ecological balance, microenvironmental climate, and environmental quality improvement. Few systematic literature have elaborated the adsorption and response mechanisms of atmospheric particulate matter by plants. We summarized the causes and composition of atmospheric particulate matter, as well as the adsorption methods and factors of plants on atmospheric particulate matter. Moreover, we elaborated the impact of atmospheric particulate matter stress on phenotypic and physiological characteristics, as well as molecular mechanisms. For the future researches, we proposed 1) to select plant species with strong adaptability and high dust retention capacity. Subsequently, there should be a universal green dust retention plan on account of comprehensive factors such as plant community structure, street morphology, and planting space; 2) to extend the research from urban areas to agricultural and pastoral areas, with a systematic analysis of the comprehensive dust retention capacity of communities with different plant configuration; 3) to effectively combine the dust retention capacity of plants with their own resistance. Subsequently, we should explore the physiological and molecular mechanisms of plants responding to atmospheric particulate matter stress and establish a comprehensive evaluation system and criteria; 4) to develop in situ labeling detection technology, which would be a valuable tool for accurately tracing and quanti-fying the dynamics of atmospheric particulate matter within plant at the cellular level.


Asunto(s)
Contaminantes Atmosféricos , Material Particulado , Plantas , Material Particulado/análisis , Plantas/metabolismo , Plantas/química , Contaminantes Atmosféricos/análisis , Adsorción , Atmósfera/química , Biodegradación Ambiental , Contaminación del Aire/análisis , Contaminación del Aire/prevención & control
16.
Environ Geochem Health ; 46(10): 415, 2024 Sep 05.
Artículo en Inglés | MEDLINE | ID: mdl-39235477

RESUMEN

Emergency ambulance dispatches (EAD) have been proven to be associated with ambient particulate matter with diameter < 2.5 µm (PM2.5) concentration, but the associations of circulatory EAD remained inconclusive, especially in heavily polluted areas. In this time series conducted in Shenyang City, Northeastern China, we explored the associations between circulatory EAD and ambient PM2.5 and its constituents. Data including 113,508 circulatory EAD records, five types of PM2.5 constituents, and meteorological information spanning from 2014 to 2019 were retrieved. Using generalized additive models (GAMs), we explored the association between circulatory EAD and calculated excess risks induced by a 10 µg/m3 increase (ERR10) in PM2.5 mass and its constituents. ERR by percentage change (ERRpc) to compare among the different constituents were also calculated. Positive associations between circulatory EAD and PM2.5 mass, sulfates, organic matters, and black carbon, were found particularly at lag0 and lag0-5, with the ERR10 of 3.8% (3.2%-4.4%), 6.5% (2.2%-10.8%), 4.2% (1.7%-6.6%), and 30.2% (17.2%-43.4%) at lag0-5, respectively. Similar associations were observed for cardiovascular EAD, while cerebrovascular EAD suggested a positive association with O3 rather than PM2.5 or its constituents. Notably, PM2.5 mass exhibited the largest ERRpc for circulatory and cardiovascular EAD, followed by sulfates and black carbon. Moreover, the risks were enhanced for circulatory and cardiovascular EAD in males compared to females and during warmer seasons compared to colder seasons. Our findings contribute new evidence on PM2.5 exposure and circulatory EAD in relatively polluted areas.


Asunto(s)
Contaminantes Atmosféricos , Ambulancias , Material Particulado , Material Particulado/análisis , Humanos , China , Contaminantes Atmosféricos/análisis , Exposición a Riesgos Ambientales , Contaminación del Aire , Femenino , Masculino , Enfermedades Cardiovasculares/epidemiología , Enfermedades Cardiovasculares/inducido químicamente
17.
JAMA Netw Open ; 7(9): e2432245, 2024 Sep 03.
Artículo en Inglés | MEDLINE | ID: mdl-39240563

RESUMEN

Importance: Ambient air pollution and antimicrobial resistance pose significant global public health challenges. It is not known whether ambient air pollution is associated with increased consumption of antimicrobials. Objective: To assess whether a short-term association exists between ambient air pollution levels and antimicrobial consumption among the general population seeking primary care consultations for acute respiratory symptoms. Design, Setting, and Participants: This 2-stage cross-sectional ecological time series analysis study using data on daily ambient air pollution and antimicrobial consumption was conducted in the 11 largest cities in Catalonia, Spain, from June 23, 2012, to December 31, 2019, among all inhabitants aged 12 years or older. Statistical analysis was performed from November 2022 to December 2023. Exposures: Daily ambient air pollution (particulate matter of 10 µg/m3 [PM10], particulate matter of 2.5 µg/m3 [PM2.5], and nitrogen dioxide [NO2]). Main Outcomes and Measures: The main outcome was antimicrobial consumption associated with primary care consultations for acute respiratory symptoms in the 30 days before and after the dispensing of the antimicrobial. Antimicrobial consumption was measured as defined daily doses (DDDs) per 1000 inhabitants per day. Results: Among 1 938 333 inhabitants (median age, 48 years [IQR, 34-65 years]; 55% female participants), there were 8 421 404 antimicrobial dispensations, with a median of 12.26 DDDs per 1000 inhabitants per day (IQR, 6.03-15.32 DDDs per 1000 inhabitants per day). The median adjusted morbidity score was 2.0 (IQR, 1.0-5.0). For the 1 924 814 antimicrobial dispensations associated with primary care consultations for acute respiratory symptoms, there was a significant correlation between increases of 10 µg/m3 in the concentration of the 3 pollutants studied and heightened antimicrobial consumption at day 0 (PM10: relative risk [RR], 1.01 [95% CI, 1.01-1.02]; PM2.5: RR, 1.03 [95% CI, 1.01-1.04]; NO2: RR, 1.04 [95% CI, 1.03-1.05]). A delayed association emerged between increases in PM2.5 concentration and antimicrobial consumption between day 7 (RR, 1.00 [95% CI, 1.00-1.01]) and day 10 (RR, 1.00 [95% CI, 1.00-1.01]) after exposure. Conclusions and Relevance: In this 2-stage cross-sectional study using ecological time series analysis, short-term exposure to air pollution was associated with increased antimicrobial use associated with primary care consultations for acute respiratory symptoms in the general population. This finding could contribute to informing policy decisions aimed at reducing air pollution and its associated risks, thereby promoting respiratory health and reducing antimicrobial use.


Asunto(s)
Contaminación del Aire , Humanos , Femenino , Masculino , Contaminación del Aire/efectos adversos , Contaminación del Aire/análisis , Persona de Mediana Edad , Estudios Transversales , Adulto , España/epidemiología , Anciano , Material Particulado/efectos adversos , Material Particulado/análisis , Antiinfecciosos/uso terapéutico , Antiinfecciosos/efectos adversos , Exposición a Riesgos Ambientales/efectos adversos , Exposición a Riesgos Ambientales/estadística & datos numéricos , Adolescente , Adulto Joven , Niño , Infecciones del Sistema Respiratorio/tratamiento farmacológico , Infecciones del Sistema Respiratorio/epidemiología
18.
Biomedica ; 44(3): 391-401, 2024 08 29.
Artículo en Inglés, Español | MEDLINE | ID: mdl-39241241

RESUMEN

Introduction: Air quality is a matter of interest for public health due to its rapid deterioration in low- and middle-income countries and the effects of polluted air on the health of populations. Objective: To explore the air quality conditions in which digital platform delivery workers carry out their work, evaluating the localities of Kennedy and Usaquén in Bogotá, 2021. Materials and methods: We developed a mixed parallel convergent study based on four sources of information: 1) Ethnographic observation in five commercial locations of the two localities; 2) Monitoring of PM10 and PM2.5 in 56 delivery routes using a low-cost sensor; 3) Daily logs of the routes to support the device data interpretation, and 4) A semi-structured interview applied to the drivers to explore their danger perception during the routes. Results: We identified elements causing environmental injustice among digital platform delivery workers between the two study locations. The routes made by the delivery drivers in the locality of Kennedy registered higher concentrations of PM10 and PM2.5, compared to the values observed in Usaquén. The sources of air pollution identified by the delivery drivers through ethnographic observation and the router logbook showed the worst parameters in Kennedy. Conclusions: We evidenced that air quality, urban equipment, road infrastructure, mobile sources, and geospatial location are elements that mark the presence of environmental injustice for the digital platform delivery drivers in the studied localities. To reduce this inequity, it is necessary for digital delivery platforms and the district government to implement strategies that reduce the exposure and emission of air pollutants to protect the health of digital platform delivery workers.


Introducción: La calidad del aire es un asunto de interés para la salud pública por su rápido deterioro en los países de bajos y medianos ingresos, y los efectos del aire contaminado en la salud de las poblaciones. Objetivo: Explorar las condiciones de la calidad del aire en las que los repartidores de plataformas digitales desarrollaron su trabajo en las localidades de Kennedy y Usaquén de Bogotá durante el 2021. Materiales y métodos: Se llevó a cabo un estudio mixto, paralelo y convergente, basado en cuatro fuentes de información: 1) observación etnográfica en cinco ubicaciones comerciales de las dos localidades; 2) monitoreo de PM10 y PM2.5 en 56 rutas de reparto, empleando un equipo de bajo costo; 3) bitácoras diarias de los recorridos que apoyaron la interpretación de los datos del equipo, y 4) entrevista semiestructurada con el rutero para explorar sus percepciones frente a los peligros durante los recorridos. Resultados: Se identificaron diferencias en las condiciones de trabajo, las percepciones y las exposiciones a material particulado de los repartidores entre las dos localidades de estudio que constituyeron fuentes de injusticia ambiental. Los recorridos que realizaron los repartidores en la localidad de Kennedy registraron mayores concentraciones de PM10 y PM2.5. Las fuentes de contaminación atmosférica identificadas por los repartidores mostraron los peores parámetros en Kennedy. Conclusiones: Se evidenció que la calidad del aire, el equipamiento urbano, la infraestructura vial, las fuentes móviles y la ubicación geoespacial son elementos que marcan la presencia de injusticia ambiental para los repartidores. Para disminuir esta inequidad, es necesario que las plataformas de reparto digital y el gobierno distrital implementen estrategias que reduzcan la exposición y la emisión de contaminantes del aire con el fin de proteger la salud de los repartidores de plataformas.


Asunto(s)
Contaminación del Aire , Material Particulado , Colombia , Humanos , Contaminación del Aire/análisis , Material Particulado/análisis , Monitoreo del Ambiente/métodos , Exposición Profesional/prevención & control , Justicia Social , Contaminantes Atmosféricos/análisis
19.
Environ Monit Assess ; 196(10): 888, 2024 Sep 04.
Artículo en Inglés | MEDLINE | ID: mdl-39230597

RESUMEN

Although low-cost air quality sensors facilitate the implementation of denser air quality monitoring networks, enabling a more realistic assessment of individual exposure to airborne pollutants, their sensitivity to multifaceted field conditions is often overlooked in laboratory testing. This gap was addressed by introducing an in-field calibration and validation of three PAQMON 1.0 mobile sensing low-cost platforms developed at the Mining and Metallurgy Institute in Bor, Republic of Serbia. A configuration tailored for monitoring PM2.5 and PM10 mass concentrations along with meteorological parameters was employed for outdoor measurement campaigns in Bor, spanning heating (HS) and non-heating (NHS) seasons. A statistically significant positive linear correlation between raw PM2.5 and PM10 measurements during both campaigns (R > 0.90, p ≤ 0.001) was observed. Measurements obtained from the uncalibrated NOVA SDS011 sensors integrated into the PAQMON 1.0 platforms exhibited a substantial and statistically significant correlation with the GRIMM EDM180 monitor (R > 0.60, p ≤ 0.001). The calibration models based on linear and Random Forest (RF) regression were compared. RF models provided more accurate descriptions of air quality, with average adjR2 values for air quality variables in the range of 0.70 to 0.80 and average NRMSE values between 0.35 and 0.77. RF-calibrated PAQMON 1.0 platforms displayed divergent levels of accuracy across different pollutant concentration ranges, achieving a data quality objective of 50% during both measurement campaigns. For PM2.5, uncertainty ( U r ) was below 50% for concentrations between 9.06 and 34.99 µg/m3 in HS and 5.75 and 17.58 µg/m3 in NHS, while for PM10, it stayed below 50% from 19.11 to 51.13 µg/m3 in HS and 11.72 to 38.86 µg/m3 in NHS.


Asunto(s)
Contaminantes Atmosféricos , Contaminación del Aire , Monitoreo del Ambiente , Aprendizaje Automático , Material Particulado , Material Particulado/análisis , Monitoreo del Ambiente/métodos , Monitoreo del Ambiente/instrumentación , Contaminantes Atmosféricos/análisis , Contaminación del Aire/estadística & datos numéricos , Serbia , Calibración
20.
Environ Monit Assess ; 196(10): 895, 2024 Sep 04.
Artículo en Inglés | MEDLINE | ID: mdl-39230792

RESUMEN

This study investigated seasonal fluctuations in particulate matter (PM) concentrations, including carbon and polycyclic aromatic hydrocarbon (PAH) components, in Phnom Penh, Cambodia, focusing on ultrafine particles (UFPs or ≤ 100 nm). UFP levels were notably higher during the dry season, averaging 23.73 ± 3.7 µg/m3 compared to 19.64 ± 3.4 µg/m3 in the wet season, attributed to increased emissions from vehicles and agricultural burning. In contrast, lower concentrations during the wet season were due to scavenging effect of rain. When compared to other Southeast Asian cities, UFP levels in Phnom Penh were significantly higher during the dry season, surpassing those in cities like Bangkok and Kuala Lumpur. Seasonal variations in carbonaceous components showed higher elemental carbon (EC) and total carbon (TC) during the dry season, with EC/TC ratios suggesting substantial influence from vehicular emissions and biomass burning. PAH analysis revealed seasonal disparities, with higher concentrations of benzo[b]fluoranthene (BbF) and benzo[k]fluoranthene (BkF) during the wet season, whereas fluoranthene (Flu) and pyrene (Pyr) were consistently present, indicating diverse PAH sources. The Flu/(Flu + Pyr) ratios, indicative of biomass burning, were higher in the dry season. Correlations between PAHs and carbon components confirmed combustion as a significant source of PAHs, aligning with global trends. This emphasizes the need to address distinct PM sources during various season in Phnom Penh.


Asunto(s)
Contaminantes Atmosféricos , Carbono , Monitoreo del Ambiente , Material Particulado , Hidrocarburos Policíclicos Aromáticos , Hidrocarburos Policíclicos Aromáticos/análisis , Cambodia , Material Particulado/análisis , Contaminantes Atmosféricos/análisis , Carbono/análisis , Emisiones de Vehículos/análisis , Estaciones del Año , Contaminación del Aire/estadística & datos numéricos , Tamaño de la Partícula , Ciudades
SELECCIÓN DE REFERENCIAS
DETALLE DE LA BÚSQUEDA