Carbamoylation of Azomethine Imines via Visible-Light Photoredox Catalysis.

Matsuo, Bianca T; Oliveira, Pedro H R; Correia, José Tiago M; Paixão, Márcio W

Matsuo, Bianca T; Oliveira, Pedro H R; Correia, José Tiago M; Paixão, Márcio W.

Afiliação

Matsuo BT; Centre of Excellence for Research in Sustainable Chemistry (CERSusChem), Department of Chemistry, Federal University of São Carlos - UFSCar, Washington Luís Highway, km 235, São Carlos, São Paulo 13565-905, Brazil.
Oliveira PHR; Centre of Excellence for Research in Sustainable Chemistry (CERSusChem), Department of Chemistry, Federal University of São Carlos - UFSCar, Washington Luís Highway, km 235, São Carlos, São Paulo 13565-905, Brazil.
Correia JTM; Centre of Excellence for Research in Sustainable Chemistry (CERSusChem), Department of Chemistry, Federal University of São Carlos - UFSCar, Washington Luís Highway, km 235, São Carlos, São Paulo 13565-905, Brazil.
Paixão MW; Centre of Excellence for Research in Sustainable Chemistry (CERSusChem), Department of Chemistry, Federal University of São Carlos - UFSCar, Washington Luís Highway, km 235, São Carlos, São Paulo 13565-905, Brazil.

Org Lett ; 23(17): 6775-6779, 2021 09 03.

Article em En | MEDLINE | ID: mdl-34428073

RESUMO

A versatile and robust photocatalytic methodology to install the amide functional group into azomethine imine ions is described. This protocol is distinguished by its broad scope and mild reaction conditions, which are well suited for the preparation of structurally complex compounds in the form of amino acids, peptides, and small drug-like molecules. Moreover, the generated pyrazolidinone core could be easily converted into ß-alanine analogues.

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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Org Lett Assunto da revista: BIOQUIMICA Ano de publicação: 2021 Tipo de documento: Article País de afiliação: Brasil País de publicação: Estados Unidos

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