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Ni2+-binding RNA motifs with an asymmetric purine-rich internal loop and a G-A base pair.
Hofmann, H P; Limmer, S; Hornung, V; Sprinzl, M.
Afiliación
  • Hofmann HP; Laboratorium für Biochemie, Universität Bayreuth, Germany.
RNA ; 3(11): 1289-300, 1997 Nov.
Article en En | MEDLINE | ID: mdl-9409620
RNA molecules with high affinity for immobilized Ni2+ were isolated from an RNA pool with 50 randomized positions by in vitro selection-amplification. The selected RNAs preferentially bind Ni2+ and Co2+ over other cations from first series transition metals. Conserved structure motifs, comprising about 15 nt, were identified that are likely to represent the Ni2+ binding sites. Two conserved motifs contain an asymmetric purine-rich internal loop and probably a mismatch G-A base pair. The structure of one of these motifs was studied with proton NMR spectroscopy and formation of the G-A pair at the junction of helix and internal loop was demonstrated. Using Ni2+ as a paramagnetic probe, a divalent metal ion binding site near this G-A base pair was identified. Ni2+ ions bound to this motif exert a specific stabilization effect. We propose that small asymmetric purine-rich loops that contain a G-A interaction may represent a divalent metal ion binding site in RNA.
Asunto(s)

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Purinas / ARN / Adenina / Guanina / Níquel Tipo de estudio: Clinical_trials Idioma: En Revista: RNA Asunto de la revista: BIOLOGIA MOLECULAR Año: 1997 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Purinas / ARN / Adenina / Guanina / Níquel Tipo de estudio: Clinical_trials Idioma: En Revista: RNA Asunto de la revista: BIOLOGIA MOLECULAR Año: 1997 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos