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Refined structure for the complex of D-gluco-dihydroacarbose with glucoamylase from Aspergillus awamori var. X100 to 2.2 A resolution: dual conformations for extended inhibitors bound to the active site of glucoamylase.
Stoffer, B; Aleshin, A E; Firsov, L M; Svensson, B; Honzatko, R B.
Afiliación
  • Stoffer B; Department of Chemistry, Carlsberg Laboratory, Copenhagen Valby, Denmark.
FEBS Lett ; 358(1): 57-61, 1995 Jan 16.
Article en En | MEDLINE | ID: mdl-7821430
The crystal structure at pH 4 of the complex of glucoamylase II(471) from Aspergillus awamori var. X100 with the pseudotetrasaccharide D-gluco-dihydroacarbose has been refined to an R-factor of 0.125 against data to 2.2 A resolution. The first two residues of the inhibitor bind at a position nearly identical to those of the closely related inhibitor acarbose in its complex with glucoamylase at pH 6. However, the electron density bifurcates beyond the second residue of the D-gluco-dihydroacarbose molecule, placing the third and fourth residues together at two positions in the active site. The position of relatively low density (estimated occupancy of 35%) corresponds to the location of the third and fourth residues of acarbose in its complex with glucoamylase at pH 6. The position of high density (65% occupancy) corresponds to a new binding mode of an extended inhibitor to the active site of glucoamylase. Presented are possible causes for the binding of D-gluco-dihydroacarbose in two conformations at the active site of glucoamylase at pH 4.
Asunto(s)
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Conformación Proteica / Aspergillus / Trisacáridos / Glucano 1,4-alfa-Glucosidasa Tipo de estudio: Prognostic_studies Idioma: En Revista: FEBS Lett Año: 1995 Tipo del documento: Article País de afiliación: Dinamarca Pais de publicación: Reino Unido
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Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Conformación Proteica / Aspergillus / Trisacáridos / Glucano 1,4-alfa-Glucosidasa Tipo de estudio: Prognostic_studies Idioma: En Revista: FEBS Lett Año: 1995 Tipo del documento: Article País de afiliación: Dinamarca Pais de publicación: Reino Unido