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Double Tips for In-Plane Polarized Near-Field Microscopy and Spectroscopy.
Kusch, Patryk; Arcos Pareja, José Andrés; Tsarapkin, Aleksei; Deinhart, Victor; Harbauer, Karsten; Hoeflich, Katja; Reich, Stephanie.
Afiliación
  • Kusch P; Freie Universität Berlin, Fachbereich Physik, Berlin, Berlin 14195, Germany.
  • Arcos Pareja JA; Freie Universität Berlin, Fachbereich Physik, Berlin, Berlin 14195, Germany.
  • Tsarapkin A; Ferdinand-Braun-Institut, Leibniz-Institut fuer Hoechstfrequenztechnik (FBH), Berlin, Berlin 12489 Germany.
  • Deinhart V; Ferdinand-Braun-Institut, Leibniz-Institut fuer Hoechstfrequenztechnik (FBH), Berlin, Berlin 12489 Germany.
  • Harbauer K; Institute for Solar Fuels, Helmholtz-Zentrum Berlin fuer Materialien und Energie GmbH, Berlin, Berlin 14109 Germany.
  • Hoeflich K; Ferdinand-Braun-Institut, Leibniz-Institut fuer Hoechstfrequenztechnik (FBH), Berlin, Berlin 12489 Germany.
  • Reich S; Freie Universität Berlin, Fachbereich Physik, Berlin, Berlin 14195, Germany.
Nano Lett ; 2024 Sep 10.
Article en En | MEDLINE | ID: mdl-39254859
ABSTRACT
Near-field optical microscopy and spectroscopy provide high-resolution imaging below the diffraction limit, crucial in physics, chemistry, and biology for studying molecules, nanoparticles, and viruses. These techniques use a sharp metallic tip of an atomic force microscope (AFM) to enhance incoming and scattered light by excited near-fields at the tip apex, leading to high sensitivity and a spatial resolution of a few nanometers. However, this restricts the near-field orientation to out-of-plane polarization, limiting optical polarization choices. We introduce double tips that offer in-plane polarization for enhanced imaging and spectroscopy. These double tips provide superior enhancement over single tips, although with a slightly lower spatial resolution (∼30 nm). They enable advanced studies of nanotubes, graphene defects, and transition metal dichalcogenides, benefiting from polarization control. The double tips allow varied polarization in tip-enhanced Raman scattering and selective excitation of transverse-electric and -magnetic polaritons, expanding the range of nanoscale samples that can be studied.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2024 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2024 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos