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Revisiting the estimation indicator for HONO emissions from light-duty vehicles.
Yang, Xinping; Fu, Mingliang; Liao, Songdi; Tu, Zhipeng; Feng, Weijie; Wang, Yunjing; Jiang, Han; Tian, Qili; Yin, Hang; Zheng, Junyu; Ding, Yan.
Afiliación
  • Yang X; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Fu M; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China. Electronic address: fumingl
  • Liao S; College of Environment and Climate, Institute for Environmental and Climate Research, Jinan University, Guangzhou 511436, China. Electronic address: sdliao@jnu.edu.cn.
  • Tu Z; College of Environment and Climate, Institute for Environmental and Climate Research, Jinan University, Guangzhou 511436, China.
  • Feng W; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Wang Y; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Jiang H; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Tian Q; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Yin H; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China; Vehicle Emission Control Center, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
  • Zheng J; Sustainable Energy and Environment Thrust, The Hong Kong University of Science and Technology (Guangzhou), Guangzhou 511458, China. Electronic address: junyuzheng@hkust-gz.edu.cn.
  • Ding Y; State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
J Hazard Mater ; 479: 135642, 2024 Nov 05.
Article en En | MEDLINE | ID: mdl-39197281
ABSTRACT
Gaseous nitrous acid (HONO), playing a crucial role in the generation of hydroxyl (OH) radicals and thus secondary pollution, lacks a source. Vehicular emission is a significant HONO source and is usually estimated by a traditional estimation indicator (RHONO/NOx = 0.8 %). Nevertheless, with more direct measurements for vehicular HONO emissions, RHONO/NOx values have been reported to vary over a wide range. In this study, we conducted the driving tests with a chassis dynamometer for ten light-duty gasoline vehicles. HONO emission factors have realized a significant reduction with the updating of emission standards, with emission factors of 0.40 mg/km, 0.13 mg/km, and 0.06 mg/km for China IV, China V, and China VI vehicles, respectively. Besides precursors, water content and exhaust temperature were found to be possible decisive factors for initiating HONO generation. Furthermore, by coupling NOx emissions and combustion efficiency, we modified the estimation indicator for vehicular HONO emissions and a better estimation effect has been verified. Additionally, we established a dynamic inventory of vehicular HONO emissions in Jinniu District in Chengdu and further found the traditional estimation indicator would overestimate HONO emissions by around 17 %. Our findings would help to advance a deeper understanding of vehicular HONO emissions and the modified estimation indicator would be beneficial in minimizing the uncertainties of the HONO budget in the troposphere.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Hazard Mater Asunto de la revista: SAUDE AMBIENTAL Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Países Bajos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: J Hazard Mater Asunto de la revista: SAUDE AMBIENTAL Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Países Bajos