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Metal-Organic Frameworks as a Thermal Emitter for High-Performance Passive Radiative Cooling.
Lam, Do Van; Dung, Dao Thi; Nguyen, Uyen Nhat Trieu; Kang, Hyun Seok; Bae, Byeong-Soo; Kim, Hyeon-Don; Lim, Mikyung; Kim, Duckjong; Kim, Jae-Hyun; Lee, Seung-Mo.
Afiliación
  • Lam DV; National Creative Research Initiative Center for Functionally Antagonistic Nano-Engineering, Department of Mechanical Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon, 34141, South Korea.
  • Dung DT; Korea Institute of Machinery and Materials (KIMM), 156 Gajeongbuk-ro, Yuseong-gu, Daejeon, 34103, South Korea.
  • Nguyen UNT; University of Science and Technology (UST), 217 Gajeong-ro, Yuseong-gu, Daejeon, 34113, South Korea.
  • Kang HS; Korea Institute of Machinery and Materials (KIMM), 156 Gajeongbuk-ro, Yuseong-gu, Daejeon, 34103, South Korea.
  • Bae BS; University of Science and Technology (UST), 217 Gajeong-ro, Yuseong-gu, Daejeon, 34113, South Korea.
  • Kim HD; Wearable Platform Materials Technology Center (WMC), Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon, 34141, South Korea.
  • Lim M; Wearable Platform Materials Technology Center (WMC), Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon, 34141, South Korea.
  • Kim D; Korea Institute of Machinery and Materials (KIMM), 156 Gajeongbuk-ro, Yuseong-gu, Daejeon, 34103, South Korea.
  • Kim JH; Korea Institute of Machinery and Materials (KIMM), 156 Gajeongbuk-ro, Yuseong-gu, Daejeon, 34103, South Korea.
  • Lee SM; School of Mechanical and Aerospace Engineering, Gyeongsang National University, 501 Jinju-daero, Jinju, Gyeongnam, 52828, South Korea.
Small Methods ; : e2401141, 2024 Aug 16.
Article en En | MEDLINE | ID: mdl-39149767
ABSTRACT
Passive radiative cooling represents a transformative approach to achieving sustainable cooling on Earth without relying on energy consumption. In this research, the optical characteristics of five readily accessible metal-organic frameworks (MOFs) ZIF-67(Co), MOF-74(Ni), HKUST-1(Cu), MOF-801(Zr), and UiO-66(Zr) are meticulously explored. The objective is to identify the pivotal factors that influence their ability to facilitate radiative cooling. Through an in-depth analysis encompassing spectroscopic features, surface texture, and porosity, it is found that the MOFs' cooling efficacy is largely influenced by their optical bandgaps and functional groups, although other factors like chemical composition and structural characteristics remain to be considered. Notably, UiO-66(Zr) emerged as the standout performer, boasting an impressive solar reflectance of 91% and a mid-infrared emissivity of 96.8%. Remarkably, a fabric treated with UiO-66(Zr) achieved a substantial sub-ambient cooling effect, lowering temperatures by up to 5 °C and delivering a cooling power of 26 W m-2 at 300 K. The findings underscore the vast potential of MOFs in offering new opportunities to advance passive radiative cooling technologies, paving the way for their extensive application in this field.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Methods Año: 2024 Tipo del documento: Article País de afiliación: Corea del Sur Pais de publicación: Alemania
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
Buscar en Google

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Methods Año: 2024 Tipo del documento: Article País de afiliación: Corea del Sur Pais de publicación: Alemania