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Micronano Lasers Based on Aggregation-Induced Emission Molecules: Diverse Resonant Cavities Investigation.
Wang, Qikai; Niu, Yi; Zhang, Shoubin; Hu, Yufeng; Lou, Zhidong; Hou, Yanbing; Zhao, Yong Sheng; Teng, Feng; Cui, Qiuhong.
Afiliación
  • Wang Q; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Niu Y; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Zhang S; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Hu Y; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Lou Z; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Hou Y; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Zhao YS; Key Laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China.
  • Teng F; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
  • Cui Q; Department of Materials Science and Engineering, School of Physical Sciences and Engineering, Beijing Jiaotong University, Beijing 100044, China.
ACS Appl Mater Interfaces ; 16(33): 44026-44032, 2024 Aug 21.
Article en En | MEDLINE | ID: mdl-39133654
ABSTRACT
Aggregation-induced emission (AIE) molecules have great potential to enhance the performance of micronano lasers due to their excellent aggregated luminescence properties, so it is valuable to expand their applications in micronano lasers. In this work, a typical AIE active fluorescent dye motif 9,10-bis(2,2-diphenylvinyl) anthracene (BDPVA) was selected as the gain medium. First, drop-casting was used to fabricate BDPVA single-crystal nanowires, which can be used as Fabry-Perot (FP)-type resonators with a lasing threshold of 49.4 µJ/cm2. Furthermore, we innovatively doped BDPVA molecules as gain mediums into external polymer Whispering-Gallery-Mode (WGM)-type resonators via the emulsion self-assembly method. Fabricated BDPVA-doped polystyrene (PS) microspheres exhibit a much lower lasing threshold of 9.04 µJ/cm2. These results prove that the BDPVA molecules, in addition to realizing the reported AIE single-crystal lasers, can also be used as a guest-doped gain medium in the resonant cavity for obtaining better fluorescence gain. In addition, multimode tunability of two types of lasers has been successfully achieved by tuning the structure of the resonant cavity. This work further expands the application potential of AIE materials and will provide a useful reference for the rational design and fabrication of photonic micronano laser components using AIE materials.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos