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Developing Cathode Films for Practical All-Solid-State Lithium-Sulfur Batteries.
Ye, Chao; Xu, Shijie; Li, Huan; Shan, Jieqiong; Qiao, Shi-Zhang.
Afiliación
  • Ye C; School of Chemical Engineering, The University of Adelaide, Adelaide, SA, 5005, Australia.
  • Xu S; School of Chemical Engineering, The University of Adelaide, Adelaide, SA, 5005, Australia.
  • Li H; School of Chemical Engineering, The University of Adelaide, Adelaide, SA, 5005, Australia.
  • Shan J; Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong, 999077, P. R. China.
  • Qiao SZ; School of Chemical Engineering, The University of Adelaide, Adelaide, SA, 5005, Australia.
Adv Mater ; : e2407738, 2024 Jul 29.
Article en En | MEDLINE | ID: mdl-39075816
ABSTRACT
The development of all-solid-state lithium-sulfur batteries (ASSLSBs) toward large-scale electrochemical energy storage is driven by the higher specific energies and lower cost in comparison with the state-of-the-art Li-ion batteries. Yet, insufficient mechanistic understanding and quantitative parameters of the key components in sulfur-based cathode hinders the advancement of the ASSLSB technologies. This review offers a comprehensive analysis of electrode parameters, including specific capacity, voltage, S mass loading and S content toward establishing the specific energy (Wh kg-1) and energy density (Wh L-1) of the ASSLSBs. Additionally, this work critically evaluates the progress in enhancing lithium ion and electron percolation and mitigating electrochemical-mechanical degradation in sulfur-based cathodes. Last, a critical outlook on potential future research directions is provided to guide the rational design of high-performance sulfur-based cathodes toward practical ASSLSBs.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Australia Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Australia Pais de publicación: Alemania