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Stimuli-responsive AIEgens with an ultra acidochromic scope for self-reporting soft actuators.
Wang, Jinjin; Wang, Xingxiao; Li, Mengzhen; Wang, Haoran; Gao, Haoyu; Zheng, Xin; Liu, Guoxing; Niu, Caoyuan; Liu, Qian; Hu, Zhiyuan; Zhou, Yuanyuan; Zhao, Zheng; Yang, Jinglei; Liu, Lijie.
Afiliación
  • Wang J; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Wang X; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Li M; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Wang H; Faculty of Materials Science, Shenzhen MSU-BIT University, Shenzhen, 518115, China.
  • Gao H; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Zheng X; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Liu G; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Niu C; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China.
  • Liu Q; Department of Urology, Tianjin First Central Hospital, Tianjin 300192, China.
  • Hu Z; Henan Engineering Research Center of Green Synthesis for Pharmaceuticals, School of Chemistry and Chemical Engineering, Shangqiu Normal University, Shangqiu 476000, China.
  • Zhou Y; School of Materials Science and Engineering, Henan Engineering Research Center of Design and Recycle for Advanced Electrochemical Energy Storage Materials, Henan Normal University, Xinxiang, 453007, China.
  • Zhao Z; School of Science and Engineering, Shenzhen Institute of Aggregate Science and Technology, The Chinese University of Hong Kong Shenzhen (CUHK-Shenzhen), Guangdong, 518172, China. Electronic address: zhaozheng@cuhk.edu.cn.
  • Yang J; Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, China. Electronic address: maeyang@ust.hk.
  • Liu L; College of Science, Henan Agricultural University, 63 Agricultural Road, Zhengzhou, Henan, 450002, China; Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, China. Electronic address: lijieliu@henau.edu.cn.
Biosens Bioelectron ; 263: 116582, 2024 Nov 01.
Article en En | MEDLINE | ID: mdl-39038401
ABSTRACT
This study develops a series of NBI-based acidochromic AIEgens engineered for ultra-wide acidochromic scope in self-reporting soft actuators, establishing the relationship between the photophysical properties and structural configurations of the AIEgens, further investigating their acidochromic behavior and fabricating acidity monitoring chips. The acidochromic behaviors were thoroughly investigated, and high-precision acidity monitoring chips were fabricated. We confirmed the protonation order of nitrogen atoms within the molecules and elucidated the acidochromic mechanisms through DFT and 1H NMR analyses. Utilizing these findings, we designed acid-driven hydrogel-based biomimetic actuators that can self-report and control the release of heavy loads under acidic conditions. These actuators hold significant potential for applications in targeted drug delivery within acidic biological environments, controlled release systems, and specialized transportation of heavy loads under acidic conditions.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Técnicas Biosensibles Idioma: En Revista: Biosens Bioelectron Asunto de la revista: BIOTECNOLOGIA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Reino Unido
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Técnicas Biosensibles Idioma: En Revista: Biosens Bioelectron Asunto de la revista: BIOTECNOLOGIA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Reino Unido