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Mechanistic insight into near-infrared light-driven Cu2O/WO2 Ohmic contact photothermal catalysts for high-efficiency antibiotic wastewater purification.
Li, Jihui; Sun, Shaodong; Lyu, Jieli; Yu, Xiaojing; Zhao, Jiaqing; Yang, Man; Yang, Bian; Yang, Qing; Cui, Jie.
Afiliación
  • Li J; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Sun S; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Lyu J; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Yu X; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Zhao J; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Yang M; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Yang B; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Yang Q; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
  • Cui J; Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education; Shaanxi Engineering Research Center of Metal-Based Heterogeneous Materials and Advanced Manufacturing Technology; Shaanxi Province Key Laboratory for Electrical Materials and Infiltration Technology;
Nanoscale ; 16(29): 14116-14129, 2024 Jul 25.
Article en En | MEDLINE | ID: mdl-39011579
ABSTRACT
Near-infrared (NIR) light-induced photothermal effect is beneficial for accelerating catalytic processes; thus, it is imperative to develop novel photothermal catalysts for promoting practical application. Herein, we synthesized NIR-responsive Cu2O/WO2 Ohmic contact photothermal catalysts through a facile ethylene glycol-assisted liquid-phase reduction method. In this photothermal catalyst, a new-type NIR-responsive Cu2O semiconductor is integrated with an NIR-responsive WO2 semimetal component to form an Ohmic contact, which is more beneficial for simultaneously promoting photocharge separation and enhancing NIR light absorption for a high-efficiency photothermal effect. As expected, the Cu2O/WO2 composite displays higher NIR light-driven photothermal catalytic performance for tetracycline removal from wastewater. Various characterization methods and density functional theory calculations were performed to obtain in-depth mechanistic insights into the NIR light-driven Cu2O/WO2 Ohmic contact photothermal catalysts. Hopefully, this research could provide a useful guideline for researchers focusing on the photothermal engineering of new composite photocatalysts.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nanoscale Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido