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Small Additives Make Big Differences: A Review on Advanced Additives for High-Performance Solid-State Li Metal Batteries.
Kim, Donggun; Hu, Xin; Yu, Baozhi; Chen, Ying Ian.
Afiliación
  • Kim D; Institute for Frontier Materials, Deakin University, Waurn Ponds, VIC, 3216, Australia.
  • Hu X; Institute for Frontier Materials, Deakin University, Waurn Ponds, VIC, 3216, Australia.
  • Yu B; Institute for Frontier Materials, Deakin University, Waurn Ponds, VIC, 3216, Australia.
  • Chen YI; Institute for Frontier Materials, Deakin University, Waurn Ponds, VIC, 3216, Australia.
Adv Mater ; 36(33): e2401625, 2024 Aug.
Article en En | MEDLINE | ID: mdl-38934341
ABSTRACT
Solid-state lithium (Li) metal batteries, represent a significant advancement in energy storage technology, offering higher energy densities and enhanced safety over traditional Li-ion batteries. However, solid-state electrolytes (SSEs) face critical challenges such as lower ionic conductivity, poor stability at the electrode-electrolyte interface, and dendrite formation, potentially leading to short circuits and battery failure. The introduction of additives into SSEs has emerged as a transformative approach to address these challenges. A small amount of additives, encompassing a range from inorganic and organic materials to nanostructures, effectively improve ionic conductivity, drawing it nearer to that of their liquid counterparts, and strengthen mechanical properties to prevent cracking of SSEs and maintain stable interfaces. Importantly, they also play a critical role in inhibiting the growth of dendritic Li, thereby enhancing the safety and extending the lifespan of the batteries. In this review, the wide variety of additives that have been investigated, is comprehensively explored, emphasizing how they can be effectively incorporated into SSEs. By dissecting the operational mechanisms of these additives, the review hopes to provide valuable insights that can help researchers in developing more effective SSEs, leading to the creation of more efficient and reliable solid-state Li metal batteries.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Australia Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Australia Pais de publicación: Alemania