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Quantification of Methane Emissions from Cold Heavy Oil Production with Sand Extraction in Alberta and Saskatchewan, Canada.
Han, Tianran; Liggio, John; Narayan, Julie; Liu, Yayong; Hayden, Katherine; Mittermeier, Richard; Darlington, Andrea; Wheeler, Michael; Cober, Stewart; Zhang, Yuheng; Xie, Conghui; Yang, Yanrong; Huang, Yufei; Wolde, Mengistu; Smyth, Steve; Barrigar, Owen; Li, Shao-Meng.
Afiliación
  • Han T; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Liggio J; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Narayan J; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Liu Y; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Hayden K; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Mittermeier R; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Darlington A; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Wheeler M; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Cober S; Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada.
  • Zhang Y; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Xie C; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Yang Y; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Huang Y; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
  • Wolde M; Flight Research Laboratory, National Research Council Canada Aerospace Research Centre, Ottawa, Ontario K1V 1J8, Canada.
  • Smyth S; Pollutant Inventories and Reporting Division, Environment and Climate Change Canada, Gatineau, Québec K1A 0H6, Canada.
  • Barrigar O; Pollutant Inventories and Reporting Division, Environment and Climate Change Canada, Gatineau, Québec K1A 0H6, Canada.
  • Li SM; State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
Environ Sci Technol ; 2024 Jun 04.
Article en En | MEDLINE | ID: mdl-38832692
ABSTRACT
Cold heavy oil production with sand (CHOPS) is an extraction process for heavy oil in Canada, with the potential to lead to higher CH4 venting than conventional oil sites, that have not been adequately characterized. In order to quantify CH4 emissions from CHOPS activities, a focused aerial measurement campaign was conducted in the Canadian provinces of Alberta and Saskatchewan in June 2018. Total CH4 emissions from each of 10 clusters of CHOPS wells (containing 22-167 well sites per cluster) were derived using a mass balance computation algorithm that uses in situ wind data measurement on board aircraft. Results show that there is no statistically significant difference in CH4 emissions from CHOPS wells between the two provinces. Cluster-aggregated emission factors (EF) were determined using correspondingly aggregated production volumes. The average CH4 EF was 70.4 ± 36.9 kg/m3 produced oil for the Alberta wells and 55.1 ± 13.7 kg/m3 produced oil for the Saskatchewan wells. Using these EF and heavy oil production volumes reported to provincial regulators, the annual CH4 emissions from CHOPS were estimated to be 121% larger than CHOPS emissions extracted from Canada's National Inventory Report (NIR) for Saskatchewan. The EF were found to be positively correlated with the percentage of nonpiped production volumes in each cluster, indicating higher emissions for nonpiped wells while suggesting an avenue for methane emission reductions. A comparison with recent measurements indicates relatively limited effectiveness of regulations for Saskatchewan compared to those in Alberta. The results of this study indicate the substantial contribution of CHOPS operations to the underreporting observed in the NIR and provide measurement-based EF that can be used to develop improved emissions inventories for this sector and mitigate CH4 emissions from CHOPS operations.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Environ Sci Technol Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Environ Sci Technol Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos