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High-Branched Natural Polysaccharide Flaxseed Gum Binder for Silicon-Based Lithium-Ion Batteries with High Capacity.
Zhou, Wenbo; Zhang, Renwei; Yu, Shijie; Peng, Zexuan; Zuo, Caixin; Yang, Wenjuan; Li, Yafeng; Wei, Mingdeng.
Afiliación
  • Zhou W; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Zhang R; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Yu S; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Peng Z; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Zuo C; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Yang W; School of Energy, Materials and Chemical Engineering, Hefei University, Hefei, 230601, China.
  • Li Y; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
  • Wei M; Fujian Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou, 350116, China.
Small ; 20(36): e2403048, 2024 Sep.
Article en En | MEDLINE | ID: mdl-38708777
ABSTRACT
Silicon-based anodes heavily depend on the binder to preserve the unbroken electrode structure. In the present work, natural flaxseed gum (FG) is used as a binder of silicon nanoparticles (SiNPs) anode for the first time. Owing to a large number of polar groups and a rich branched structure, this material not only anchors tightly to the surface of SiNPs through bonding interactions but also formed a hydrogen bonding network structure among molecules. As a result, the FG binder can endow the silicon electrode with stable interfacial adhesion and outstanding mechanical properties. In addition, FG with a high viscosity facilitates the homogeneous dispersion of the electrode components. When FG is used as a binder, the cycling performance of the Si anode is greatly improved. After one hundred cycles at an applied current density of 1 A g-1, the electrode continues to display remarkable electrochemical properties with a significant cyclic capacity (2213 mA h g-1) and initial Coulombic efficiency (ICE) of 89.7%.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Asunto de la revista: ENGENHARIA BIOMEDICA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Asunto de la revista: ENGENHARIA BIOMEDICA Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Alemania