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Local incomplete combustion emissions define the PM2.5 oxidative potential in Northern India.
Bhattu, Deepika; Tripathi, Sachchida Nand; Bhowmik, Himadri Sekhar; Moschos, Vaios; Lee, Chuan Ping; Rauber, Martin; Salazar, Gary; Abbaszade, Gülcin; Cui, Tianqu; Slowik, Jay G; Vats, Pawan; Mishra, Suneeti; Lalchandani, Vipul; Satish, Rangu; Rai, Pragati; Casotto, Roberto; Tobler, Anna; Kumar, Varun; Hao, Yufang; Qi, Lu; Khare, Peeyush; Manousakas, Manousos Ioannis; Wang, Qiyuan; Han, Yuemei; Tian, Jie; Darfeuil, Sophie; Minguillon, Mari Cruz; Hueglin, Christoph; Conil, Sébastien; Rastogi, Neeraj; Srivastava, Atul Kumar; Ganguly, Dilip; Bjelic, Sasa; Canonaco, Francesco; Schnelle-Kreis, Jürgen; Dominutti, Pamela A; Jaffrezo, Jean-Luc; Szidat, Sönke; Chen, Yang; Cao, Junji; Baltensperger, Urs; Uzu, Gaëlle; Daellenbach, Kaspar R; El Haddad, Imad; Prévôt, André S H.
Afiliación
  • Bhattu D; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland. dbhattu@iitj.ac.in.
  • Tripathi SN; Department of Civil and Infrastructure Engineering, Indian Institute of Technology Jodhpur, Rajasthan, India. dbhattu@iitj.ac.in.
  • Bhowmik HS; Department of Civil Engineering & Department of Sustainable Energy Engineering, Indian Institute of Technology Kanpur, Uttar Pradesh, India. snt@iitk.ac.in.
  • Moschos V; Department of Sustainable Energy Engineering, Indian Institute of Technology Kanpur, Uttar Pradesh, India. snt@iitk.ac.in.
  • Lee CP; Department of Civil Engineering & Department of Sustainable Energy Engineering, Indian Institute of Technology Kanpur, Uttar Pradesh, India.
  • Rauber M; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Salazar G; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Abbaszade G; Department of Chemistry, Biochemistry and Pharmaceutical Sciences, University of Bern, Bern, Switzerland.
  • Cui T; Oeschger Centre for Climate Change Research, University of Bern, Bern, Switzerland.
  • Slowik JG; Department of Chemistry, Biochemistry and Pharmaceutical Sciences, University of Bern, Bern, Switzerland.
  • Vats P; Oeschger Centre for Climate Change Research, University of Bern, Bern, Switzerland.
  • Mishra S; Comprehensive Molecular Analytics (CMA), Department Environmental Health, Helmholtz Zentrum München, Neuherberg, Germany.
  • Lalchandani V; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Satish R; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Rai P; Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India.
  • Casotto R; Department of Civil Engineering & Department of Sustainable Energy Engineering, Indian Institute of Technology Kanpur, Uttar Pradesh, India.
  • Tobler A; Department of Civil Engineering & Department of Sustainable Energy Engineering, Indian Institute of Technology Kanpur, Uttar Pradesh, India.
  • Kumar V; Geosciences Division, Physical Research Laboratory, Ahmedabad, India.
  • Hao Y; College of Engineering, Science, Technology and Agriculture, Central State University, Wilberforce, Ohio, USA.
  • Qi L; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Khare P; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Manousakas MI; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Wang Q; Datalystica Ltd., Park innovAARE, Villigen, Switzerland.
  • Han Y; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Tian J; Department of Environmental science, Aarhus University, Roskilde, Denmark.
  • Darfeuil S; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Minguillon MC; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Hueglin C; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Conil S; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Rastogi N; Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China.
  • Srivastava AK; Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China.
  • Ganguly D; Institute of Earth Environment, Chinese Academy of Sciences, Xi'an, China.
  • Bjelic S; University Grenoble Alpes, IRD, CNRS, INRAE, Grenoble INP*, IGE (Institute of Environmental Geosciences), Grenoble, France.
  • Canonaco F; Institute of Environmental Assessment and Water Research (IDAEA-CSIC), Barcelona, Spain.
  • Schnelle-Kreis J; Laboratory for Air Pollution and Environmental Technology, Swiss Federal Laboratories for Materials Science and Technology (Empa), Duebendorf, Switzerland.
  • Dominutti PA; ANDRA DRD/GES Observatoire Pérenne de l'Environnement, Bure, France.
  • Jaffrezo JL; Geosciences Division, Physical Research Laboratory, Ahmedabad, India.
  • Szidat S; Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, New Delhi, India.
  • Chen Y; Centre for Atmospheric Sciences, Indian Institute of Technology Delhi, New Delhi, India.
  • Cao J; Biogenergy and Catalysis Laboratory, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Baltensperger U; Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, Switzerland.
  • Uzu G; Datalystica Ltd., Park innovAARE, Villigen, Switzerland.
  • Daellenbach KR; Comprehensive Molecular Analytics (CMA), Department Environmental Health, Helmholtz Zentrum München, Neuherberg, Germany.
  • El Haddad I; University Grenoble Alpes, IRD, CNRS, INRAE, Grenoble INP*, IGE (Institute of Environmental Geosciences), Grenoble, France.
  • Prévôt ASH; University Grenoble Alpes, IRD, CNRS, INRAE, Grenoble INP*, IGE (Institute of Environmental Geosciences), Grenoble, France.
Nat Commun ; 15(1): 3517, 2024 Apr 25.
Article en En | MEDLINE | ID: mdl-38664406
ABSTRACT
The oxidative potential (OP) of particulate matter (PM) is a major driver of PM-associated health effects. In India, the emission sources defining PM-OP, and their local/regional nature, are yet to be established. Here, to address this gap we determine the geographical origin, sources of PM, and its OP at five Indo-Gangetic Plain sites inside and outside Delhi. Our findings reveal that although uniformly high PM concentrations are recorded across the entire region, local emission sources and formation processes dominate PM pollution. Specifically, ammonium chloride, and organic aerosols (OA) from traffic exhaust, residential heating, and oxidation of unsaturated vapors from fossil fuels are the dominant PM sources inside Delhi. Ammonium sulfate and nitrate, and secondary OA from biomass burning vapors, are produced outside Delhi. Nevertheless, PM-OP is overwhelmingly driven by OA from incomplete combustion of biomass and fossil fuels, including traffic. These findings suggest that addressing local inefficient combustion processes can effectively mitigate PM health exposure in northern India.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2024 Tipo del documento: Article País de afiliación: Suiza Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nat Commun Asunto de la revista: BIOLOGIA / CIENCIA Año: 2024 Tipo del documento: Article País de afiliación: Suiza Pais de publicación: Reino Unido