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Supercritical water oxidation for the treatment and utilization of organic wastes: Factor effects, reaction enhancement, and novel process.
Li, Yanhui; Duan, Yuanwang; Wang, Shuzhong; Zhang, Fan; Li, Jianna; Dai, Zheng; Li, Zicheng; Zhang, Yishu; Wang, Yulong.
Afiliación
  • Li Y; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China. Electronic address: yhli19@sina.com.
  • Duan Y; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
  • Wang S; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China. Electronic address: szwang@aliyun.com.
  • Zhang F; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
  • Li J; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
  • Dai Z; Xi'AN University of Science and Technology, College of Safety Science and Engineering, Xi'an, Shaanxi, 710054, China.
  • Li Z; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
  • Zhang Y; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
  • Wang Y; Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, No. 28 Xianning West Road, Xi'an, 710049, China.
Environ Res ; 251(Pt 1): 118571, 2024 Jun 15.
Article en En | MEDLINE | ID: mdl-38431066
ABSTRACT
Supercritical water oxidation (SCWO) has been regarded as a new and efficient technology for the harmless treatment and energy utilization of organic wastes, resulting in the quickly homogeneous oxidation between organics and oxidizers and the former being wholly degraded into small environment-friendly green molecules such as H2O and N2 and inorganic salts. This paper systematically analyzed the influencing behavior and mechanisms of the reaction factors, such as temperature, pressure, residence time, oxidant type, oxidation coefficient, and the concentration and pH values of the raw material, on the treatment effect of organic wastes. For most organic wastes, the SCWO conditions at 550 °C with a residence time of 1min and an oxidation coefficient of 100% can meet the removal rate of more than 99%. To further enhance the degradation rate of organics, the principles, implementation cases, and related equipment components of general enhancement technologies of supercritical water oxidation were discussed, such as fractional oxygen injection, auxiliary fuel co-oxidation, and hydrothermal flame-assisted degradation. This paper proposes a novel supercritical flame-assisted oxidation process in which the reactor performs preheating, corrosion protection, and desalination functions. The use of additive-enhanced oxidation, segmented oxidation, and supercritical hydrothermal flame-assisted oxidation has achieved good results in the complicated treatment process of brutal degradation of organic matter.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Oxidación-Reducción / Agua Idioma: En Revista: Environ Res Año: 2024 Tipo del documento: Article Pais de publicación: Países Bajos
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
Buscar en Google

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Oxidación-Reducción / Agua Idioma: En Revista: Environ Res Año: 2024 Tipo del documento: Article Pais de publicación: Países Bajos