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Juice Vesicles Bioreactors Technology for Constructing Advanced Carbon-Based Energy Storage.
Shen, Shenghui; Chen, Yanbin; Gu, Xinyi; Chen, Ketong; Qiu, Zhong; Liu, Ping; Zhang, Yongqi; Xiang, Jiayuan; Yang, Yefeng; Cao, Feng; Wang, Chen; Wan, Wangjun; He, Xinping; Liang, Xinqi; Bao, Ningzhong; Chen, Minghua; Xia, Yang; Xia, Xinhui; Zhang, Wenkui.
Afiliación
  • Shen S; School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
  • Chen Y; College of Materials Science & Engineering, Zhejiang University of Technology, Hangzhou, 310014, P. R. China.
  • Gu X; School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310027, P. R. China.
  • Chen K; Narada Powder Source Co. Ltd., Hangzhou, 310014, P. R. China.
  • Qiu Z; State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering, Nanjing Tech University, Nanjing, Jiangsu, 210009, P. R. China.
  • Liu P; School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
  • Zhang Y; School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
  • Xiang J; School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
  • Yang Y; Institute of Fundamental and Frontier Science, University of Electronic Science and Technology of China, Chengdu, 611371, P. R. China.
  • Cao F; College of Materials Science & Engineering, Zhejiang University of Technology, Hangzhou, 310014, P. R. China.
  • Wang C; School of Materials Science and Engineering, Zhejiang University, Hangzhou, 310027, P. R. China.
  • Wan W; Institute of Fundamental and Frontier Science, University of Electronic Science and Technology of China, Chengdu, 611371, P. R. China.
  • He X; Narada Powder Source Co. Ltd., Hangzhou, 310014, P. R. China.
  • Liang X; School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, P. R. China.
  • Bao N; Department of Engineering Technology, Huzhou College, Huzhou, 313000, P. R. China.
  • Chen M; Zhejiang Academy of Science and Technology for Inspection & Quarantine, Hangzhou, 311215, P. R. China.
  • Xia Y; Zhejiang Academy of Science and Technology for Inspection & Quarantine, Hangzhou, 311215, P. R. China.
  • Xia X; College of Materials Science & Engineering, Zhejiang University of Technology, Hangzhou, 310014, P. R. China.
  • Zhang W; Institute of Fundamental and Frontier Science, University of Electronic Science and Technology of China, Chengdu, 611371, P. R. China.
Adv Mater ; 36(24): e2400245, 2024 Jun.
Article en En | MEDLINE | ID: mdl-38377331
ABSTRACT
The construction of high-quality carbon-based energy materials through biotechnology has always been an eager goal of the scientific community. Herein, juice vesicles bioreactors (JVBs) bio-technology based on hesperidium (e.g., pomelo, waxberry, oranges) is first reported for preparation of carbon-based composites with controllable components, adjustable morphologies, and sizes. JVBs serve as miniature reaction vessels that enable sophisticated confined chemical reactions to take place, ultimately resulting in the formations of complex carbon composites. The newly developed approach is highly versatile and can be compatible with a wide range of materials including metals, alloys, and metal compounds. The growth and self-assembly mechanisms of carbon composites via JVBs are explained. For illustration, NiCo alloy nanoparticles are successfully in situ implanted into pomelo vesicles crosslinked carbon (PCC) by JVBs, and their applications as sulfur/carbon cathodes for lithium-sulfur batteries are explored. The well-designed PCC/NiCo-S electrode exhibits superior high-rate properties and enhanced long-term stability. Synergistic reinforcement mechanisms on transportation of ions/electrons of interface reactions and catalytic conversion of lithium polysulfides arising from metal alloy and carbon architecture are proposed with the aid of DFT calculations. The research provides a novel biosynthetic route to rational design and fabrication of carbon composites for advanced energy storage.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article Pais de publicación: Alemania
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
Buscar en Google

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2024 Tipo del documento: Article Pais de publicación: Alemania