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Switchable surface and loading/release of target molecules in hierarchically porous PLA nonwovens based on shape memory effect.
Zhang, Lishuo; Chai, Wenqiang; Zhang, Jiaru; Chen, Zhouli; Yue, Ziyang; Wang, Jiayao; Yu, Jiankang.
Afiliación
  • Zhang L; College of Safety Science and Engineering, Liaoning Technical University Huludao 125105 China.
  • Chai W; College of Material, Chemistry and Chemical Engineering, Hangzhou Normal University Hangzhou 311121 China Jiayao-wang@outlook.com.
  • Zhang J; Tongxiang Jianmin Filter Material Product Co. LTD. 314511 Jiaxing China.
  • Chen Z; College of Material, Chemistry and Chemical Engineering, Hangzhou Normal University Hangzhou 311121 China Jiayao-wang@outlook.com.
  • Yue Z; Zhejiang Institute of Mechanical & Electrical Engineering Hangzhou 311203 China xiaoliu1018@126.com.
  • Wang J; College of Science, Liaoning Technical University Fuxin 123000 China 13591995463@163.com.
  • Yu J; College of Material, Chemistry and Chemical Engineering, Hangzhou Normal University Hangzhou 311121 China Jiayao-wang@outlook.com.
RSC Adv ; 14(9): 6199-6204, 2024 Feb 14.
Article en En | MEDLINE | ID: mdl-38375019
ABSTRACT
In this work, hierarchically porous PLA (polylactic acid) shape memory nonwovens were prepared by electrospinning its blend solution with PEO (polyethylene oxide) and subsequent water etching. Based on shape memory effect resulting from tiny crystals and the amorphous matrix of PLA, the switch between compact and porous surfaces has been achieved via cyclical hot-pressing and recovery in a hot water bath. After hot-pressing, the disappearance of hierarchical pores contributes to compact surface, enabling embedding of the target molecule in PLA nonwoven (i.e., CLOSE state). Upon exposure to heat, PLA nonwoven recovers to its permanent shape and exhibits a porous surface, providing a penetrative diffusion pathway for small molecules (i.e., OPEN state). The hierarchically porous structure and shape memory effect endow PLA nonwoven with the capability of rapid release. Our results provide a good candidate for some potential applications, such as temperature-controlled quick-release of catalysts and drugs.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2024 Tipo del documento: Article Pais de publicación: Reino Unido