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Opportunity and challenges in recovering and functionalizing anode graphite from spent lithium-ion batteries: A review.
Gao, Yang; Zhang, Shaoyan; Lin, Shuanglong; Li, Zhongqiu; Chen, Yongqiang; Wang, Chengyan.
Afiliación
  • Gao Y; Shijiazhuang Key Laboratory of Low Carbon Energy Materials, College of Chemical Engineering, Shijiazhuang University, Shijiazhuang, Hebei, 050035, China.
  • Zhang S; Shijiazhuang Key Laboratory of Low Carbon Energy Materials, College of Chemical Engineering, Shijiazhuang University, Shijiazhuang, Hebei, 050035, China. Electronic address: zsyedu@hotmail.com.
  • Lin S; Shijiazhuang Key Laboratory of Low Carbon Energy Materials, College of Chemical Engineering, Shijiazhuang University, Shijiazhuang, Hebei, 050035, China.
  • Li Z; Shijiazhuang Key Laboratory of Low Carbon Energy Materials, College of Chemical Engineering, Shijiazhuang University, Shijiazhuang, Hebei, 050035, China; Shijiazhuang Concrete Green Intelligent Manufacturing and Recycling Technology Innovation Center, Shijiazhuang, Hebei, 050035, China.
  • Chen Y; State Key Laboratory of Advanced Metallurgy, University of Science and Technology Beijing, Beijing, 100083, China; School of Metallurgical and Ecological Engineering, University of Science and Technology Beijing, Beijing, 100083, China.
  • Wang C; State Key Laboratory of Advanced Metallurgy, University of Science and Technology Beijing, Beijing, 100083, China; School of Metallurgical and Ecological Engineering, University of Science and Technology Beijing, Beijing, 100083, China. Electronic address: chywang@yeah.net.
Environ Res ; 247: 118216, 2024 Apr 15.
Article en En | MEDLINE | ID: mdl-38242420
ABSTRACT
Recent concerns have emerged regarding the improper disposal of spent lithium-ion batteries (LIBs), which has garnered widespread societal attention. Graphite materials accounted for 12-21 wt % of LIBs' mass, typically contain heavy metals, binders, and residual electrolytes. Regenerating spent graphite not only alleviated the shortage of plumbago, but also contributed to the supports environmental protection as well as national carbon peak and neutrality ("dual carbon" goals). Despite significant advancements in recycling spent LIBs had been made, a comprehensive overview of the processes for pretreatment, regeneration, and functionalization of spent graphite from retired LIBs, along with the associated technical standards and industry regulations enabling their smooth implementation still needed to be mentioned. Hence, we conducted the following research work. Firstly, the pre-treatment process of spent graphite, including discharging, crushing, and screening was summed up. Next,. Subsequently, graphite recovery methods, such as acid leaching, pyrometallurgy, and combined methods were summarized. Moreover, the modification and doping approach was used to enhance the electrochemical properties of graphite. Afterwards, we reviewed the functionalization of anode graphite from an economically and environmentally friendly view. Meanwhile, the technical standards and industry regulations of spent LIBs in domestic and oversea industries were described. Finally, we provided an overview of the technical challenges and development bottlenecks in graphite recycling, along with future prospects Overall, this study outlined the opportunities and challenges in recovering and functionalizing of anode materials via a efficient and sustainable processes.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Grafito / Litio Tipo de estudio: Guideline Idioma: En Revista: Environ Res Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Países Bajos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Grafito / Litio Tipo de estudio: Guideline Idioma: En Revista: Environ Res Año: 2024 Tipo del documento: Article País de afiliación: China Pais de publicación: Países Bajos