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Enhancing composite electrode performance: insights into interfacial interactions.
Ren, Haoze; Takeuchi, Esther S; Marschilok, Amy C; Takeuchi, Kenneth J; Reichmanis, Elsa.
Afiliación
  • Ren H; Department of Chemical and Bimolecular Engineering, Lehigh University, Bethlehem, PA, 18015, USA. elr420@lehigh.edu.
  • Takeuchi ES; Interdisciplinary Science Department, Brookhaven National Laboratory, Upton, New York, 11973, USA.
  • Marschilok AC; Institute for Energy Sustainability, Environment and Equity, Stony Brook University, Stony Brook, New York, 11794, USA.
  • Takeuchi KJ; Department of Material Science and Chemical Engineering, Stony Brook University, Stony Brook, New York, 11794, USA.
  • Reichmanis E; Department of Chemistry, Stony Brook University, Stony Brook, New York, 11794, USA.
Chem Commun (Camb) ; 60(15): 1979-1998, 2024 Feb 15.
Article en En | MEDLINE | ID: mdl-38190114
ABSTRACT
Propelled by the widespread adoption of portable electronic devices, electrochemical energy storage systems, particularly lithium-ion batteries (LIBs), have become ubiquitous in modern society. The electrode is the critical battery component, where intricate interactions between the materials govern both the energy output and the overall lifespan of the battery under operational conditions. However, the poor interfacial properties of traditional electrode materials fall short in meeting escalating performance demands. To facilitate the advent of next-generation lithium-ion batteries, attention must be devoted to the interfacial chemistry that dictates and modulates the various dynamic and transport processes across multiple length scales within the composite electrodes. Recent research has concentrated on systematically understanding the properties of distinct electrode components to engineer meticulously tailored electrode formulations. These are geared towards composite electrodes with heightened chemical stability, thermal robustness, enhanced local conductivities, and superior mechanical resilience. This review elucidates the latest advances in understanding the impact of interfacial interactions in achieving high-capacity, high-stability electrodes. Through comprehensive insights into the interfacial interactions between the various electrode components, we can create improved integrated systems that outperform those developed through empirical methods. In light of this, the adoption of a holistic approach to enhance the interactions among electrode materials becomes of paramount importance. This concerted effort ensures the attainment of heightened rate capability, facilitation of lithium-ion transport, and overall system stability throughout the entirety of the cyclic process.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
Buscar en Google

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2024 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Reino Unido