Phonon Signatures in Photon Correlations.

Humphries, Ben S; Green, Dale; Borgh, Magnus O; Jones, Garth A

Humphries, Ben S; Green, Dale; Borgh, Magnus O; Jones, Garth A.

Afiliación

Humphries BS; School of Chemistry, University of East Anglia, Norwich Research Park, Norwich, NR4 7TJ, United Kingdom.
Green D; School of Chemistry, University of East Anglia, Norwich Research Park, Norwich, NR4 7TJ, United Kingdom.
Borgh MO; Physics, Faculty of Science, University of East Anglia, Norwich NR4 7TJ, United Kingdom.
Jones GA; School of Chemistry, University of East Anglia, Norwich Research Park, Norwich, NR4 7TJ, United Kingdom.

Phys Rev Lett ; 131(14): 143601, 2023 Oct 06.

Article en En | MEDLINE | ID: mdl-37862651

RESUMEN

We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and antibunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems.

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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Phys Rev Lett Año: 2023 Tipo del documento: Article País de afiliación: Reino Unido Pais de publicación: Estados Unidos

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