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Enhanced Electromechanical Performance in Lead-free (Na,K)NbO3-Based Piezoceramics via the Synergistic Design of Texture Engineering and Sm-Modification.
Liu, Yang; Shen, Bingzhong; Bian, Lang; Hao, Jigong; Yang, Bin; Zhang, Rui; Cao, Wenwu.
Afiliación
  • Liu Y; Functional Materials and Acousto-optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China.
  • Shen B; Functional Materials and Acousto-optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China.
  • Bian L; Functional Materials and Acousto-optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China.
  • Hao J; School of Materials Science and Engineering, Liaocheng University, Liaocheng 252059, China.
  • Yang B; Functional Materials and Acousto-optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China.
  • Zhang R; Functional Materials and Acousto-optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China.
  • Cao W; Department of Mathematics and Materials Research Institute, The Pennsylvania State University, University Park, Pennsylvania 16802, United States.
ACS Appl Mater Interfaces ; 15(40): 47221-47228, 2023 Oct 11.
Article en En | MEDLINE | ID: mdl-37768723
Next-generation electromechanical conversion devices have a significant demand for high-performance lead-free piezoelectric materials to meet environmentally friendly requirements. However, the low electromechanical properties of lead-free piezoceramics limit their application in high-end transducer applications. In this work, a 0.96K0.48Na0.52Nb0.96Sb0.04O3-0.04(Bi0.5-xSmx)Na0.5ZrO3 (abbreviated as T-NKN-xSm) ceramic was designed through phase regulation and texture engineering, which is expected to solve this difficulty. Through our research, we successfully demonstrated the enhanced electromechanical performance of lead-free textured ceramics with a highly oriented [001]c orientation. Notably, the T-NKN-xSm textured ceramics doped with 0.05 mol % Sm exhibited the optimal electromechanical performance: piezoelectric coefficient d33 ≈ 710 pC N-1, longitudinal electromechanical coupling k33 ≈ 0.88, planar electromechanical coupling kp ≈ 0.80, and Curie temperature Tc ≈ 244 °C. Finally, we conducted a detailed investigation into the phase and domain structures of the T-NKN-Sm ceramics, providing valuable insights for achieving high electromechanical properties in NKN-based ceramics. This research serves as a crucial reference for the development of advanced electromechanical devices by facilitating the utilization of lead-free piezoelectric materials with superior performance and environmental benefits.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2023 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2023 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos