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SERS-substrates based on ZnO nanoflowers prepared by green synthesis.
Dzhagan, Volodymyr; Smirnov, Oleksandr; Kovalenko, Mariia; Gudymenko, Oleksandr; Mazur, Nazar; Kapush, Olga; Skoryk, Mykola; Pirko, Yaroslav; Yemets, Alla; Valakh, Mykhailo; Shepeliavyi, Petro; Yukhymchuk, Volodymyr.
Afiliación
  • Dzhagan V; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine; Physics Department, Taras Shevchenko National University of Kyiv, Kyiv, Ukraine. Electronic address: dzhagan@isp.kiev.ua.
  • Smirnov O; ESC "Institute of Biology and Medicine", Taras Shevchenko National University of Kyiv, Kyiv, Ukraine; Institute of Plant Physiology and Genetics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Kovalenko M; ESC "Institute of Biology and Medicine", Taras Shevchenko National University of Kyiv, Kyiv, Ukraine.
  • Gudymenko O; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Mazur N; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Kapush O; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Skoryk M; G.V. Kurdyumov Institute for Metal Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Pirko Y; Institute of Food Biotechnology and Genomics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Yemets A; Institute of Food Biotechnology and Genomics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Valakh M; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Shepeliavyi P; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
  • Yukhymchuk V; V. Lashkaryov Institute of Semiconductors Physics, National Academy of Sciences of Ukraine, Kyiv, Ukraine.
Anal Biochem ; 681: 115328, 2023 Nov 15.
Article en En | MEDLINE | ID: mdl-37722524
ZnO nanoparticles (NPs) with a flower-like morphology, synthesized by an affordable colloidal route using an aqueous fungi extract of Ganoderma lucidum as a reducing agent and stabilizer, are investigated as SERS-substrate. Each "flower" has large effective surface that is preserved at packing particles into a dense film and thus exhibits an advantageous property for SERS and similar sensing applications. The mycoextract used in our low-cost and green synthesis as surface stabilizer allows subsequent deposition of metal NPs or layers. One type of SERS substrates studied here was ZnO NPs decorated in situ in the solution by Ag NPs, another type was prepared by thermally evaporating Ag layer on the ZnO NP film on a substrate. A huge difference in the enhancement of the same analyte in the solution and in the dried form is found and discussed. Detection down to 10-7 M of standard dye analytes such as rhodamine 6G and methylene blue was achieved without additional optimization of the SERS substrates. The observed SERS-activity demonstrate the potential of both the free-standing flower-like ZnO NPs and thereof made dense films also for other applications where large surface area accessible for the external agent is crucial, such as catalysis or sensing.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Anal Biochem Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Anal Biochem Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos