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Scaffold Morphing and In Silico Design of Potential BACE-1 (ß-Secretase) Inhibitors: A Hope for a Newer Dawn in Anti-Alzheimer Therapeutics.
Bhatia, Shiveena; Singh, Manjinder; Sharma, Pratibha; Mujwar, Somdutt; Singh, Varinder; Mishra, Krishna Kumar; Singh, Thakur Gurjeet; Singh, Tanveer; Ahmad, Sheikh Fayaz.
Afiliación
  • Bhatia S; Chitkara College of Pharmacy, Chitkara University, Rajpura 140401, Punjab, India.
  • Singh M; Chitkara College of Pharmacy, Chitkara University, Rajpura 140401, Punjab, India.
  • Sharma P; Chitkara College of Pharmacy, Chitkara University, Rajpura 140401, Punjab, India.
  • Mujwar S; Chitkara College of Pharmacy, Chitkara University, Rajpura 140401, Punjab, India.
  • Singh V; Department of Pharmaceutical Sciences and Technology, Maharaja Ranjit Singh Punjab Technical University, Bathinda 151001, Punjab, India.
  • Mishra KK; Chitkara University Institute of Engineering and Technology, Chitkara University, Rajpura 140401, Punjab, India.
  • Singh TG; Chitkara College of Pharmacy, Chitkara University, Rajpura 140401, Punjab, India.
  • Singh T; Department of Neuroscience and Experimental Therapeutics, College of Medicine, Texas A&M Health Science Center, College Station, TX 77807, USA.
  • Ahmad SF; Department of Pharmacology and Toxicology, College of Pharmacy, King Saud University, Riyadh 11451, Saudi Arabia.
Molecules ; 28(16)2023 Aug 12.
Article en En | MEDLINE | ID: mdl-37630283
Alzheimer's disease (AD) is the prime cause of 65-80% of dementia cases and is caused by plaque and tangle deposition in the brain neurons leading to brain cell degeneration. ß-secretase (BACE-1) is a key enzyme responsible for depositing extracellular plaques made of ß-amyloid protein. Therefore, efforts are being applied to develop novel BACE-1 enzyme inhibitors to halt plaque build-up. In our study, we analyzed some Elenbecestat analogues (a BACE-1 inhibitor currently in clinical trials) using a structure-based drug design and scaffold morphing approach to achieve a superior therapeutic profile, followed by in silico studies, including molecular docking and pharmacokinetics methodologies. Among all the designed compounds, SB306 and SB12 showed good interactions with the catalytic dyad motifs (Asp228 and Asp32) of the BACE-1 enzyme with drug-likeliness properties and a high degree of thermodynamic stability confirmed by the molecular dynamic and stability of the simulated system indicating the inhibitory nature of the SB306 and SB12 on BACE 1.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Secretasas de la Proteína Precursora del Amiloide / Enfermedad de Alzheimer Límite: Humans Idioma: En Revista: Molecules Asunto de la revista: BIOLOGIA Año: 2023 Tipo del documento: Article País de afiliación: India Pais de publicación: Suiza

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Secretasas de la Proteína Precursora del Amiloide / Enfermedad de Alzheimer Límite: Humans Idioma: En Revista: Molecules Asunto de la revista: BIOLOGIA Año: 2023 Tipo del documento: Article País de afiliación: India Pais de publicación: Suiza