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Fabrication of reusable probe impregnated polymer monolithic sensor for the visual detection of Cd2+ in natural waters and cigarette samples.
Pedugu Sivaraman, Sushmitha; Krishna Kumar, Sangeetha; Srinivasan, Prabhakaran; Madhu, Deepan Kumar; Kancharlapalli Chinaraga, Pitchaiah; Nagarajan, Sivaraman; C V S Rao, Brahmmananda; Deivasigamani, Prabhakaran; Mohan, Akhila Maheswari.
Afiliación
  • Pedugu Sivaraman S; Department of Chemistry, School of Advanced Sciences, Vellore Institute of Technology (VIT), Vellore 632014, Tamil Nadu, India.
  • Krishna Kumar S; Department of Chemistry, School of Advanced Sciences, Vellore Institute of Technology (VIT), Vellore 632014, Tamil Nadu, India.
  • Srinivasan P; Department of Chemistry, School of Advanced Sciences, Vellore Institute of Technology (VIT), Vellore 632014, Tamil Nadu, India.
  • Madhu DK; Department of Chemistry, K. Ramakrishnan College of Technology, Samayapuram, Tiruchirappalli 621112, Tamil Nadu, India.
  • Kancharlapalli Chinaraga P; Fuel Chemistry Division, Materials Chemistry and Metal Fuel Cycle Group, Indira Gandhi Centre for Atomic Research (IGCAR), Kalpakkam 603102, Tamil Nadu, India.
  • Nagarajan S; Fuel Chemistry Division, Materials Chemistry and Metal Fuel Cycle Group, Indira Gandhi Centre for Atomic Research (IGCAR), Kalpakkam 603102, Tamil Nadu, India.
  • C V S Rao B; Fuel Chemistry Division, Materials Chemistry and Metal Fuel Cycle Group, Indira Gandhi Centre for Atomic Research (IGCAR), Kalpakkam 603102, Tamil Nadu, India.
  • Deivasigamani P; Department of Chemistry, School of Advanced Sciences, Vellore Institute of Technology (VIT), Vellore 632014, Tamil Nadu, India. Electronic address: prabhakaran.d@vit.ac.in.
  • Mohan AM; Department of Chemistry, School of Advanced Sciences, Vellore Institute of Technology (VIT), Vellore 632014, Tamil Nadu, India. Electronic address: akhila.maheswari@vit.ac.in.
J Hazard Mater ; 459: 132248, 2023 Oct 05.
Article en En | MEDLINE | ID: mdl-37595465
This work demonstrates the fabrication of a simple, low-cost naked-eye colorimetric solid-state sensor model for selective sensing of Cd2+. The sensor was developed using a polymer monolithic architect; namely, poly(n-allylthiourea-co-ethyleneglycol dimethacrylate) (poly(ATU-co-EGD) imbued with the chromophoric probe, 3-(quinoline-8-yldiazenyl)quinoline-2,4-diol (QYQD). The concocted indigenous perforated structural assemblies were studied through various microscopic, spectroscopic, and diffraction techniques. The template possessed a uniform arrangement of interconnected macro/mesoporous networks available for the maximum hooking of the QYQD probe moieties for the rapid and enhanced Cd2+ sensing process. The developed sensor offered an enhanced solid-state color transition response from yellow to dark meron for a proportional concentration increase of Cd2+ exhibiting precise absorption spectra with λmax at 475 nm. The relative stoichiometric binding ratio of the QYQD probe with Cd2+ was observed to be 2:1. The enhanced working conditions of the developed poly(ATU-co-EGD)QYQD sensor were tuned by validating various analytical conditions. The sensor exhibited a linear response signal from 2 to 150 ppb of Cd2+, and the corresponding LOD and LOQ values were 0.31 and 1.03 ppb, respectively. The efficacious performance drive of the sensor was validated in real water and cigarette samples that showed excellent data accuracy with a recovery value of ≥ 99.72% (n = 3).
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Diagnostic_studies Idioma: En Revista: J Hazard Mater Asunto de la revista: SAUDE AMBIENTAL Año: 2023 Tipo del documento: Article País de afiliación: India Pais de publicación: Países Bajos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Tipo de estudio: Diagnostic_studies Idioma: En Revista: J Hazard Mater Asunto de la revista: SAUDE AMBIENTAL Año: 2023 Tipo del documento: Article País de afiliación: India Pais de publicación: Países Bajos