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Giant Energy Density via Mechanically Tailored Relaxor Ferroelectric Behavior of PZT Thick Film.
Peddigari, Mahesh; Wang, Bo; Wang, Rui; Yoon, Woon-Ha; Jang, Jongmoon; Lee, Hyunjong; Song, Kyung; Hwang, Geon-Tae; Wang, Kai; Hou, Yuchen; Palneedi, Haribabu; Yan, Yongke; Choi, Han Seung; Wang, Jianjun; Talluri, Aravindkrishna; Chen, Long-Qing; Priya, Shashank; Jeong, Dae-Yong; Ryu, Jungho.
Afiliación
  • Peddigari M; Department of Functional Ceramics, Korea Institute of Materials Science (KIMS), Changwon, Gyeongnam, 51508, Republic of Korea.
  • Wang B; Department of Physics, Indian Institute of Technology Hyderabad, Kandi, Telangana, 502284, India.
  • Wang R; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Yoon WH; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Jang J; Department of Functional Ceramics, Korea Institute of Materials Science (KIMS), Changwon, Gyeongnam, 51508, Republic of Korea.
  • Lee H; Department of Functional Ceramics, Korea Institute of Materials Science (KIMS), Changwon, Gyeongnam, 51508, Republic of Korea.
  • Song K; Department of Materials Analysis and Evaluation, Korea Institute of Materials Science (KIMS), Changwon, Gyeongnam, 51508, Republic of Korea.
  • Hwang GT; Department of Materials Analysis and Evaluation, Korea Institute of Materials Science (KIMS), Changwon, Gyeongnam, 51508, Republic of Korea.
  • Wang K; Department of Materials Science and Engineering, Pukyong National University, Busan, 43241, Republic of Korea.
  • Hou Y; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Palneedi H; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Yan Y; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Choi HS; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Wang J; School of Materials Science and Engineering, Yeungnam University, Gyeongsan, Gyeongbuk, 38541, Republic of Korea.
  • Talluri A; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Chen LQ; Department of Physics, Indian Institute of Technology Hyderabad, Kandi, Telangana, 502284, India.
  • Priya S; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Jeong DY; Materials Research Institute/Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, 16802, USA.
  • Ryu J; Department of Materials Science and Engineering, Inha University, Incheon, 22212, Republic of Korea.
Adv Mater ; 35(45): e2302554, 2023 Nov.
Article en En | MEDLINE | ID: mdl-37406283
Relaxor ferroelectrics (RFEs) are being actively investigated for energy-storage applications due to their large electric-field-induced polarization with slim hysteresis and fast energy charging-discharging capability. Here, a novel nanograin engineering approach based upon high kinetic energy deposition is reported, for mechanically inducing the RFE behavior in a normal ferroelectric Pb(Zr0.52 Ti0.48 )O3 (PZT), which results in simultaneous enhancement in the dielectric breakdown strength (EDBS ) and polarization. Mechanically transformed relaxor thick films with 4 µm thickness exhibit an exceptional EDBS of 540 MV m-1 and reduced hysteresis with large unsaturated polarization (103.6 µC cm-2 ), resulting in a record high energy-storage density of 124.1 J cm-3 and a power density of 64.5 MW cm-3 . This fundamental advancement is correlated with the generalized nanostructure design that comprises nanocrystalline phases embedded within the amorphous matrix. Microstructure-tailored ferroelectric behavior overcomes the limitations imposed by traditional compositional design methods and provides a feasible pathway for realization of high-performance energy-storage materials.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2023 Tipo del documento: Article Pais de publicación: Alemania
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Adv Mater Asunto de la revista: BIOFISICA / QUIMICA Año: 2023 Tipo del documento: Article Pais de publicación: Alemania