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Imaging via Correlation of X-Ray Fluorescence Photons.
Trost, Fabian; Ayyer, Kartik; Prasciolu, Mauro; Fleckenstein, Holger; Barthelmess, Miriam; Yefanov, Oleksandr; Dresselhaus, J Lukas; Li, Chufeng; Bajt, Sasa; Carnis, Jerome; Wollweber, Tamme; Mall, Abhishek; Shen, Zhou; Zhuang, Yulong; Richter, Stefan; Karl, Sebastian; Cardoch, Sebastian; Patra, Kajwal Kumar; Möller, Johannes; Zozulya, Alexey; Shayduk, Roman; Lu, Wei; Brauße, Felix; Friedrich, Bertram; Boesenberg, Ulrike; Petrov, Ilia; Tomin, Sergey; Guetg, Marc; Madsen, Anders; Timneanu, Nicusor; Caleman, Carl; Röhlsberger, Ralf; von Zanthier, Joachim; Chapman, Henry N.
Afiliación
  • Trost F; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Ayyer K; Max Planck Institute for the Structure and Dynamics of Matter, 22607, Hamburg, Germany.
  • Prasciolu M; The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
  • Fleckenstein H; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Barthelmess M; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Yefanov O; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Dresselhaus JL; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Li C; The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
  • Bajt S; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Carnis J; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Wollweber T; The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
  • Mall A; Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607, Hamburg, Germany.
  • Shen Z; Max Planck Institute for the Structure and Dynamics of Matter, 22607, Hamburg, Germany.
  • Zhuang Y; The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
  • Richter S; Max Planck Institute for the Structure and Dynamics of Matter, 22607, Hamburg, Germany.
  • Karl S; Max Planck Institute for the Structure and Dynamics of Matter, 22607, Hamburg, Germany.
  • Cardoch S; Max Planck Institute for the Structure and Dynamics of Matter, 22607, Hamburg, Germany.
  • Patra KK; Department of Physics, Friedrich-Alexander-Universität Erlangen-Nürnberg, Staudtstrasse 1, 91058 Erlangen, Germany.
  • Möller J; Erlangen Graduate School in Advanced Optical Technologies (SAOT), Friedrich-Alexander Universität Erlangen-Nürnberg, Paul-Gordan-Str. 6, 91052, Erlangen, Germany.
  • Zozulya A; Department of Physics, Friedrich-Alexander-Universität Erlangen-Nürnberg, Staudtstrasse 1, 91058 Erlangen, Germany.
  • Shayduk R; Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala SE-75120, Sweden.
  • Lu W; Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala SE-75120, Sweden.
  • Brauße F; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Friedrich B; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Boesenberg U; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Petrov I; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Tomin S; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Guetg M; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Madsen A; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Timneanu N; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Caleman C; Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany.
  • Röhlsberger R; Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany.
  • von Zanthier J; European X-Ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
  • Chapman HN; Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala SE-75120, Sweden.
Phys Rev Lett ; 130(17): 173201, 2023 Apr 28.
Article en En | MEDLINE | ID: mdl-37172237
We demonstrate that x-ray fluorescence emission, which cannot maintain a stationary interference pattern, can be used to obtain images of structures by recording photon-photon correlations in the manner of the stellar intensity interferometry of Hanbury Brown and Twiss. This is achieved utilizing femtosecond-duration pulses of a hard x-ray free-electron laser to generate the emission in exposures comparable to the coherence time of the fluorescence. Iterative phasing of the photon correlation map generated a model-free real-space image of the structure of the emitters. Since fluorescence can dominate coherent scattering, this may enable imaging uncrystallised macromolecules.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Phys Rev Lett Año: 2023 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos
Texto completo
Añadir a Mi BVS
Imprimir
XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Phys Rev Lett Año: 2023 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos