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Proton Transfer Dynamics-Mediated CO2 Electroreduction.
Chen, Shanyong; Li, Xiaoqing; Li, Hongmei; Chen, Kejun; Luo, Tao; Fu, Junwei; Liu, Kang; Wang, Qiyou; Zhu, Mingshan; Liu, Min.
Afiliación
  • Chen S; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Li X; Guangdong Key Laboratory of Environmental Pollution and Health, School of Environment, Jinan University, 511443, Guangzhou, P. R. China.
  • Li H; Hunan Provincial Key Laboratory of Micro & Nano Materials Interface Science, College of Chemistry and Chemical Engineering, Central South University, 410083, Changsha, P. R. China.
  • Chen K; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Luo T; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Fu J; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Liu K; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Wang Q; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Zhu M; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
  • Liu M; Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, State Key Laboratory of Powder Metallurgy, School of Physical and Electronics, Central South University, 410083, Changsha, P. R. China.
ChemSusChem ; 16(12): e202202251, 2023 Jun 22.
Article en En | MEDLINE | ID: mdl-36820747
Electrochemical CO2 reduction reaction (CO2 RR) is crucial to addressing environmental crises and producing chemicals. Proton activation and transfer are essential in CO2 RR. To date, few research reviews have focused on this process and its effect on catalytic performance. Recent studies have demonstrated ways to improve CO2 RR by regulating proton transfer dynamics. This Concept highlights the use of regulating proton transfer dynamics to enhance CO2 RR for the target product and discusses modulation strategies for proton transfer dynamics and operative mechanisms in typical systems, including single-atom catalysts, molecular catalysts, metal heterointerfaces, and organic-ligand modified metal catalysts. Characterization methods for proton transfer dynamics during CO2 RR are also discussed, providing powerful tools for the hydrogen-involving electrochemical study. This Concept offers new insights into the CO2 RR mechanism and guides the design of efficient CO2 RR systems.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Protones / Dióxido de Carbono Idioma: En Revista: ChemSusChem Asunto de la revista: QUIMICA / TOXICOLOGIA Año: 2023 Tipo del documento: Article Pais de publicación: Alemania
Texto completo
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Imprimir
XML
PubMed Links
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Protones / Dióxido de Carbono Idioma: En Revista: ChemSusChem Asunto de la revista: QUIMICA / TOXICOLOGIA Año: 2023 Tipo del documento: Article Pais de publicación: Alemania