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Self-Powered Disinfection Using Triboelectric, Conductive Wires of Metal-Organic Frameworks.
Huo, Zheng-Yang; Yang, Yuxin; Jeong, Jang-Mook; Wang, Xiaoxiong; Zhang, He; Wei, Mingdeng; Dai, Keren; Xiong, Peixun; Kim, Sang-Woo.
Afiliación
  • Huo ZY; School of Environment and Natural Resources, Renmin University of China, Beijing 100872, People's Republic of China.
  • Yang Y; School of Advanced Materials Science and Engineering, Sungkyunkwan University (SKKU) Suwon 16419, Republic of Korea.
  • Jeong JM; School of Mechanical Engineering, Nanjing University of Science and Technology, Nanjing 210094, People's Republic of China.
  • Wang X; School of Advanced Materials Science and Engineering, Sungkyunkwan University (SKKU) Suwon 16419, Republic of Korea.
  • Zhang H; Department of Chemical and Environmental Engineering, Yale University, New Haven, Connecticut 06520-8286, United States.
  • Wei M; School of Mechanical Engineering, Nanjing University of Science and Technology, Nanjing 210094, People's Republic of China.
  • Dai K; Fujian Provincial Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fuzhou 350002, People's Republic of China.
  • Xiong P; School of Advanced Materials Science and Engineering, Sungkyunkwan University (SKKU) Suwon 16419, Republic of Korea.
  • Kim SW; School of Mechanical Engineering, Nanjing University of Science and Technology, Nanjing 210094, People's Republic of China.
Nano Lett ; 23(7): 3090-3097, 2023 Apr 12.
Article en En | MEDLINE | ID: mdl-36802718
Efficient water disinfection is vitally needed in rural and disaster-stricken areas lacking power supplies. However, conventional water disinfection methods strongly rely on external chemical input and reliable electricity. Herein, we present a self-powered water disinfection system using synergistic hydrogen peroxide (H2O2) assisted electroporation mechanisms driven by triboelectric nanogenerators (TENGs) that harvest electricity from the flow of water. The flow-driven TENG, assisted by power management systems, generates a controlled output with aimed voltages to drive a conductive metal-organic framework nanowire array for effective H2O2 generation and electroporation. The injured bacteria caused by electroporation can be further damaged by facile diffused H2O2 molecules at high throughput. A self-powered disinfection prototype enables complete disinfection (>99.9999% removal) over a wide range of flows up to 3.0 × 104 L/(m2 h) with low water flow thresholds (200 mL/min; ∼20 rpm). This rapid, self-powered water disinfection method is promising for pathogen control.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos