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Using heparan sulfate octadecasaccharide (18-mer) as a multi-target agent to protect against sepsis.
Liao, Yi-En; Xu, Yongmei; Arnold, Katelyn; Zhang, Fuming; Li, Jine; Sellers, Rani; Yin, Chaoyin; Pagadala, Vijayakanth; Inman, Anna Marie; Linhardt, Robert J; Xu, Ding; Pawlinski, Rafal; Liu, Jian.
Afiliación
  • Liao YE; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
  • Xu Y; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
  • Arnold K; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
  • Zhang F; Department of Chemistry and Chemical Biology, Center for Biotechnology and Interdisciplinary Studies, Rensselaer Polytechnic Institute, Troy, NY 12180.
  • Li J; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
  • Sellers R; Department of Pathology and Laboratory Medicine, School of Medicine, University of North Carolina, Chapel Hill, NC 27599.
  • Yin C; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
  • Pagadala V; Glycan Therapeutics Corporation, Raleigh, NC 27606.
  • Inman AM; Glycan Therapeutics Corporation, Raleigh, NC 27606.
  • Linhardt RJ; Department of Chemistry and Chemical Biology, Center for Biotechnology and Interdisciplinary Studies, Rensselaer Polytechnic Institute, Troy, NY 12180.
  • Xu D; Department of Oral Biology, School of Dental Medicine, The State University of New York at Buffalo, Buffalo, NY 14215.
  • Pawlinski R; Division of Hematology, Department of Medicine, Blood Research Center, University of North Carolina, Chapel Hill, NC 27599.
  • Liu J; Division of Chemical Biology and Medicinal Chemistry, Eshelman School of Pharmacy, University of North Carolina, Chapel Hill, NC 27599.
Proc Natl Acad Sci U S A ; 120(4): e2209528120, 2023 01 24.
Article en En | MEDLINE | ID: mdl-36649428
Sepsis is a lethal syndrome manifested by an unregulated, overwhelming inflammation from the host in response to infection. Here, we exploit the use of a synthetic heparan sulfate octadecasaccharide (18-mer) to protect against sepsis. The 18-mer not only inhibits the pro-inflammatory activity of extracellular histone H3 and high mobility group box 1 (HMGB1), but also elicits the anti-inflammatory effect from apolipoprotein A-I (ApoA-I). We demonstrate that the 18-mer protects against sepsis-related injury and improves survival in cecal ligation and puncture mice and reduces inflammation in an endotoxemia mouse model. The 18-mer neutralizes the cytotoxic histone-3 (H3) through direct interaction with the protein. Furthermore, the 18-mer enlists the actions of ApoA-I to dissociate the complex of HMGB1 and lipopolysaccharide, a toxic complex contributing to cell death and tissue damage in sepsis. Our study provides strong evidence that the 18-mer mitigates inflammatory damage in sepsis by targeting numerous mediators, setting it apart from other potential therapies with a single target.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Sepsis / Endotoxemia / Proteína HMGB1 Límite: Animals Idioma: En Revista: Proc Natl Acad Sci U S A Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Sepsis / Endotoxemia / Proteína HMGB1 Límite: Animals Idioma: En Revista: Proc Natl Acad Sci U S A Año: 2023 Tipo del documento: Article Pais de publicación: Estados Unidos