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Three-Input Logic AND Gate Drives Sequential Three-Step Catalysis by Parallel Activation of H+ and Ag+ as a Catalyst Duo.
Kundu, Sohom; Mondal, Debabrata; Rajasekaran, Vishnu Verman; Goswami, Abir; Schmittel, Michael.
Afiliación
  • Kundu S; Center of Micro- and Nanochemistry and (Bio)Technology, Department of Chemistry-Biology, Organische Chemie I, University of Siegen, Adolf-Reichwein Strasse 2, D-57068 Siegen, Germany.
  • Mondal D; Center of Micro- and Nanochemistry and (Bio)Technology, Department of Chemistry-Biology, Organische Chemie I, University of Siegen, Adolf-Reichwein Strasse 2, D-57068 Siegen, Germany.
  • Rajasekaran VV; Center of Micro- and Nanochemistry and (Bio)Technology, Department of Chemistry-Biology, Organische Chemie I, University of Siegen, Adolf-Reichwein Strasse 2, D-57068 Siegen, Germany.
  • Goswami A; Center of Micro- and Nanochemistry and (Bio)Technology, Department of Chemistry-Biology, Organische Chemie I, University of Siegen, Adolf-Reichwein Strasse 2, D-57068 Siegen, Germany.
  • Schmittel M; Center of Micro- and Nanochemistry and (Bio)Technology, Department of Chemistry-Biology, Organische Chemie I, University of Siegen, Adolf-Reichwein Strasse 2, D-57068 Siegen, Germany.
Inorg Chem ; 61(43): 17007-17011, 2022 Oct 31.
Article en En | MEDLINE | ID: mdl-36264551
Boolean operations with multiple catalysts as output are yet unknown using molecular logic. The issue is solved using a two-component ensemble, composed of a receptor and rotaxane, which acts as a three-input AND gate with a dual catalytic output. Actuation of the ensemble gate by the stoichiometric addition of metal ions (Ag+ and Cd2+) and 2,2,2-trifluoroacetic acid generated in the (1,1,1) truth table state a catalyst duo that synergistically enabled a three-step reaction, furnishing a dihydroisoquinoline as the output of a three-input logic AND gate operation.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Lógica Idioma: En Revista: Inorg Chem Año: 2022 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos
Texto completo
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XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Lógica Idioma: En Revista: Inorg Chem Año: 2022 Tipo del documento: Article País de afiliación: Alemania Pais de publicación: Estados Unidos