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Synthesis of a Zr4(embonate)6-cobalt based superstructure for photocatalytic hydrogen production.
Teng, Qian; He, Yan-Ping; Chen, Shu-Mei; Zhang, Jian.
Afiliación
  • Teng Q; State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, P. R. China. hyp041@163.com.
  • He YP; College of Chemistry, Fuzhou University, Fuzhou, Fujian 350108, China.
  • Chen SM; State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, P. R. China. hyp041@163.com.
  • Zhang J; College of Chemistry, Fuzhou University, Fuzhou, Fujian 350108, China.
Dalton Trans ; 51(31): 11612-11616, 2022 Aug 09.
Article en En | MEDLINE | ID: mdl-35852398
Herein, we report an efficient method to construct cage-based MOF materials with exposed metal active sites for catalysis. By employing Zr4L6 (L = embonate) cages as precursors for assembly with N-containing ligands and Co2+ ions, a new Zr4L6-Co based chain structure (PTC-318) has been generated through two-step reactions. Interestingly, in the absence of a photosensitizer, PTC-318 exhibits notable photocatalytic activity for H2 evolution under visible-light irradiation.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Dalton Trans Asunto de la revista: QUIMICA Año: 2022 Tipo del documento: Article Pais de publicación: Reino Unido
Texto completo
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Dalton Trans Asunto de la revista: QUIMICA Año: 2022 Tipo del documento: Article Pais de publicación: Reino Unido