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Aqueous lubrication and wear properties of nonionic bottle-brush polymers.
Moon, Hwi Hyun; Choi, Eun Jung; Yun, Sang Ho; Kim, Youn Chul; Premkumar, Thathan; Song, Changsik.
Afiliación
  • Moon HH; Department of Chemistry, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea tprem@skku.edu songcs@skku.edu.
  • Choi EJ; Department of Chemistry, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea tprem@skku.edu songcs@skku.edu.
  • Yun SH; Department of Chemistry, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea tprem@skku.edu songcs@skku.edu.
  • Kim YC; Department of Chemical Engineering, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea.
  • Premkumar T; Department of Chemistry, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea tprem@skku.edu songcs@skku.edu.
  • Song C; The University College, Sungkyunkwan University Suwon Gyeonggi 16419 Republic of Korea.
RSC Adv ; 12(28): 17740-17746, 2022 Jun 14.
Article en En | MEDLINE | ID: mdl-35765345
The usage of aqueous lubricants in eco-friendly bio-medical friction systems has attracted significant attention. Several bottle-brush polymers with generally ionic functional groups have been developed based on the structure of biological lubricant lubricin. However, hydrophilic nonionic brush polymers have attracted less attention, especially in terms of wear properties. We developed bottle-brush polymers (BP) using hydrophilic 2-hydroxyethyl methacrylate (HEMA), a highly biocompatible yet nonionic molecule. The lubrication properties of polymer films were analyzed in an aqueous state using a ball-on-disk, which revealed that BPHEMA showed a lower aqueous friction coefficient than linear poly(HEMA), even lower than hyaluronic acid (HA) and polyvinyl alcohol (PVA), which are widely used as lubricating polymers. Significantly, we discovered that the combination of HA, PVA, and BPHEMA is demonstrated to be essential in influencing the surface wear properties; the ratio of 1 : 2 (HA : BPHEMA) had the maximum wear resistance, despite a slight increase in the aqueous friction coefficient.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2022 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2022 Tipo del documento: Article Pais de publicación: Reino Unido