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Magnetically responsive polycaprolactone nanocarriers for application in the biomedical field: magnetic hyperthermia, magnetic resonance imaging, and magnetic drug delivery.
Szczech, Marta; Orsi, Davide; Lopuszynska, Natalia; Cristofolini, Luigi; Jasinski, Krzysztof; Weglarz, Wladyslaw P; Albertini, Franca; Kereïche, Sami; Szczepanowicz, Krzysztof.
Afiliación
  • Szczech M; Jerzy Haber Institute of Catalysis and Surface Chemistry, Polish Academy of Sciences Krakow Poland ncszczep@cyf-kr.edu.pl +48-124251923 +48-126395121.
  • Orsi D; Department of Mathematical, Physical and Computer Sciences, University of Parma Parma Italy.
  • Lopuszynska N; Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences Krakow Poland.
  • Cristofolini L; Department of Mathematical, Physical and Computer Sciences, University of Parma Parma Italy.
  • Jasinski K; Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences Krakow Poland.
  • Weglarz WP; Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences Krakow Poland.
  • Albertini F; Institute of Materials for Electronics and Magnetism, National Research Council (CNR) Parma Italy.
  • Kereïche S; Institute of Biology and Medical Genetics, First Faculty of Medicine, Charles University Prague Czech Republic.
  • Szczepanowicz K; Jerzy Haber Institute of Catalysis and Surface Chemistry, Polish Academy of Sciences Krakow Poland ncszczep@cyf-kr.edu.pl +48-124251923 +48-126395121.
RSC Adv ; 10(71): 43607-43618, 2020 Nov 27.
Article en En | MEDLINE | ID: mdl-35519668
There are huge demands on multifunctional nanocarriers to be used in nanomedicine. Herein, we present a simple and efficient method for the preparation of multifunctional magnetically responsive polymeric-based nanocarriers optimized for biomedical applications. The hybrid delivery system is composed of drug-loaded polymer nanoparticles (poly(caprolactone), PCL) coated with a multilayer shell of polyglutamic acid (PGA) and superparamagnetic iron oxide nanoparticles (SPIONs), which are known as bio-acceptable components. The PCL nanocarriers with a model anticancer drug (Paclitaxel, PTX) were formed by the spontaneous emulsification solvent evaporation (SESE) method, while the magnetically responsive multilayer shell was formed via the layer-by-layer (LbL) method. As a result, we obtained magnetically responsive polycaprolactone nanocarriers (MN-PCL NCs) with an average size of about 120 nm. Using the 9.4 T preclinical magnetic resonance imaging (MRI) scanner we confirmed, that obtained MN-PCL NCs can be successfully used as a MRI-detectable drug delivery system. The magnetic hyperthermia effect of the MN-PCL NCs was demonstrated by applying a 25 mT radio-frequency (f = 429 kHz) alternating magnetic field. We found a Specific Absorption Rate (SAR) of 55 W g-1. The conducted research fulfills the first step of investigation for biomedical application, which is mandatory for the planning of any in vitro and in vivo studies.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2020 Tipo del documento: Article Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: RSC Adv Año: 2020 Tipo del documento: Article Pais de publicación: Reino Unido