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Short-chain branched sulfosuccinate as a missing link between surfactants and hydrotropes.
Stemplinger, Simon; Causse, Jérémy; Prévost, Sylvain; Pellet-Rostaing, Stéphane; Zemb, Thomas; Horinek, Dominik.
Afiliación
  • Stemplinger S; ICSM, CEA, CNRS, Univ Montpellier, ENSCM, Marcoule, France.
  • Causse J; Institut für Physikalische und Theoretische Chemie, Universität Regensburg, Regensburg, Germany. Simon.Stemplinger@ur.de.
  • Prévost S; ICSM, CEA, CNRS, Univ Montpellier, ENSCM, Marcoule, France.
  • Pellet-Rostaing S; Institut Laue-Langevin, Grenoble, France.
  • Zemb T; ICSM, CEA, CNRS, Univ Montpellier, ENSCM, Marcoule, France.
  • Horinek D; ICSM, CEA, CNRS, Univ Montpellier, ENSCM, Marcoule, France.
Phys Chem Chem Phys ; 24(18): 11353-11361, 2022 May 11.
Article en En | MEDLINE | ID: mdl-35485971
Surfactants aggregate in water into micelles, and these micelles incorporate organic substances to solubilize them. Hydrotropes are compounds that increase the solubility of hydrophobic substances in water without this form of aggregation. Decreasing the chain length of the classical surfactant Aerosol OT (AOT) from C8 to C5 results in a molecule with intermediate properties. Molecular dynamics simulations and surface tension measurements are performed on this short chain derivative of AOT. This compound shows high solubility and at the same time progressive weak aggregation. The hydration of head groups hinders significant plunging into a hydrophobic core, which leads to well defined liquid chain nanodomains. The transition to bicontinuous aggregates is in the concentration range of 1 mol L-1. The sulfonate group of the head groups (placed at the water interface of worm-like aggregates) rather than the aggregate-aggregate interaction is responsible for the unusual small angle X-ray scattering pattern.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Phys Chem Chem Phys Asunto de la revista: BIOFISICA / QUIMICA Año: 2022 Tipo del documento: Article País de afiliación: Francia Pais de publicación: Reino Unido

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Phys Chem Chem Phys Asunto de la revista: BIOFISICA / QUIMICA Año: 2022 Tipo del documento: Article País de afiliación: Francia Pais de publicación: Reino Unido