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Synthesis and evaluation of novel HER-2 inhibitors to exert anti-breast cancer ability through epithelial-mesenchymal transition (EMT) pathway.
Li, Xin-Yang; Qian, Xin-Hua; Zhu, Ju; Li, Yu-Heng; Lin, Qi-Qi; Li, Shuai; Xue, Wen-Han; Jian, Ling-Yan; Meng, Fan-Hao.
Afiliación
  • Li XY; School of Pharmacy, China Medical University, Shenyang, 110122, PR China; Department of Pharmacy, Shengjing Hospital of China Medical University, Shenyang, 110004, PR China.
  • Qian XH; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Zhu J; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Li YH; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Lin QQ; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Li S; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Xue WH; School of Pharmacy, China Medical University, Shenyang, 110122, PR China.
  • Jian LY; Department of Pharmacy, Shengjing Hospital of China Medical University, Shenyang, 110004, PR China.
  • Meng FH; School of Pharmacy, China Medical University, Shenyang, 110122, PR China. Electronic address: fhmeng@cmu.edu.cn.
Eur J Med Chem ; 237: 114325, 2022 Jul 05.
Article en En | MEDLINE | ID: mdl-35452936
Human epidermal growth factor receptor 2 (HER-2) is an essential member of the receptor tyrosine kinase (RTK) superfamily and has been reported as a critical method for treating HER-2 positive breast cancer. Here, we retained (E)-4-methyl-2-(4-(trifluoromethyl)styryl)oxazole, a fragment of HER-2 inhibitor Mubritinib, and synthesized 32 novel compounds from it. We screened out the most potential compound Q7j with HER-2 positive breast cancer cells through MTT assays, which possessed low toxicity on normal cells (MCF7-10A). Subsequently, wound healing, transwell, western blotting, and immunofluorescence experiments were performed, and it was found that compound Q7j could suppress cell migration by inhibiting the phosphorylation of HER-2 and affecting the expression of EMT-related proteins. Moreover, the SKBR3 orthotopic xenograft model confirmed that compound Q7j was more effective than Mubritinib in inhibiting the proliferation of cancer cells. In general, compound Q7j was a potential HER-2 inhibitor in treating breast cancer, which may be of great significance for developing and improving HER-2 small molecule inhibitors.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Neoplasias de la Mama / Transición Epitelial-Mesenquimal Tipo de estudio: Prognostic_studies Límite: Female / Humans Idioma: En Revista: Eur J Med Chem Año: 2022 Tipo del documento: Article Pais de publicación: Francia

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Neoplasias de la Mama / Transición Epitelial-Mesenquimal Tipo de estudio: Prognostic_studies Límite: Female / Humans Idioma: En Revista: Eur J Med Chem Año: 2022 Tipo del documento: Article Pais de publicación: Francia