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Engineering Interlayer Electron-Phonon Coupling in WS2/BN Heterostructures.
Li, Yifei; Zhang, Xiaowei; Wang, Jinhuan; Ma, Xiaoli; Shi, Jin-An; Guo, Xiangdong; Zuo, Yonggang; Li, Ruijie; Hong, Hao; Li, Ning; Xu, Kai; Huang, Xinyu; Tian, Huifeng; Yang, Ying; Yao, Zhixin; Liao, PeiChi; Li, Xiao; Guo, Junjie; Huang, Yuang; Gao, Peng; Wang, Lifen; Yang, Xiaoxia; Dai, Qing; Wang, EnGe; Liu, Kaihui; Zhou, Wu; Yu, Xiaohui; Liang, Liangbo; Jiang, Ying; Li, Xin-Zheng; Liu, Lei.
Afiliación
  • Li Y; School of Materials Science and Engineering, Peking University, Beijing 100871, People's Republic of China.
  • Zhang X; International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Wang J; State Key Laboratory for Artificial Microstructure and Mesoscopic Physics, Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Ma X; State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, Collaborative Innovation Center of Quantum Matter, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Shi JA; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, People's Republic of China.
  • Guo X; School of Physical Sciences, CAS Key Laboratory of Vacuum Physics, University of Chinese Academy of Sciences, Beijing 100049, People's Republic of China.
  • Zuo Y; CAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, People's Republic of China.
  • Li R; The Key Laboratory of Unconventional Metallurgy, Ministry of Education, Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, People's Republic of China.
  • Hong H; School of Materials Science and Engineering, Peking University, Beijing 100871, People's Republic of China.
  • Li N; State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, Collaborative Innovation Center of Quantum Matter, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Xu K; International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Huang X; Electron Microscopy Laboratory, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Tian H; School of Physical Sciences, CAS Key Laboratory of Vacuum Physics, University of Chinese Academy of Sciences, Beijing 100049, People's Republic of China.
  • Yang Y; Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, People's Republic of China.
  • Yao Z; School of Materials Science and Engineering, Peking University, Beijing 100871, People's Republic of China.
  • Liao P; Center for Quantum Transport and Thermal Energy Science, School of Physics and Technology, Nanjing Normal University, Nanjing 210023, People's Republic of China.
  • Li X; School of Materials Science and Engineering, Peking University, Beijing 100871, People's Republic of China.
  • Guo J; Key Laboratory of Interface Science and Engineering in Advanced Materials, Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, People's Republic of China.
  • Huang Y; School of Materials Science and Engineering, Peking University, Beijing 100871, People's Republic of China.
  • Gao P; Center for Quantum Transport and Thermal Energy Science, School of Physics and Technology, Nanjing Normal University, Nanjing 210023, People's Republic of China.
  • Wang L; Key Laboratory of Interface Science and Engineering in Advanced Materials, Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, People's Republic of China.
  • Yang X; Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, People's Republic of China.
  • Dai Q; International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Wang E; Electron Microscopy Laboratory, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Liu K; Interdisciplinary Institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials, Peking University, Beijing 100871, People's Republic of China.
  • Zhou W; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, People's Republic of China.
  • Yu X; Songshan Lake Materials Laboratory, Dongguan 523808, People's Republic of China.
  • Liang L; CAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, People's Republic of China.
  • Jiang Y; CAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, People's Republic of China.
  • Li XZ; International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, People's Republic of China.
  • Liu L; Interdisciplinary Institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials, Peking University, Beijing 100871, People's Republic of China.
Nano Lett ; 22(7): 2725-2733, 2022 Apr 13.
Article en En | MEDLINE | ID: mdl-35293751
In van der Waals (vdW) heterostructures, the interlayer electron-phonon coupling (EPC) provides one unique channel to nonlocally engineer these elementary particles. However, limited by the stringent occurrence conditions, the efficient engineering of interlayer EPC remains elusive. Here we report a multitier engineering of interlayer EPC in WS2/boron nitride (BN) heterostructures, including isotope enrichments of BN substrates, temperature, and high-pressure tuning. The hyperfine isotope dependence of Raman intensities was unambiguously revealed. In combination with theoretical calculations, we anticipate that WS2/BN supercells could induce Brillouin-zone-folded phonons that contribute to the interlayer coupling, leading to a complex nature of broad Raman peaks. We further demonstrate the significance of a previously unexplored parameter, the interlayer spacing. By varying the temperature and high pressure, we effectively manipulated the strengths of EPC with on/off capabilities, indicating critical thresholds of the layer-layer spacing for activating and strengthening interlayer EPC. Our findings provide new opportunities to engineer vdW heterostructures with controlled interlayer coupling.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2022 Tipo del documento: Article Pais de publicación: Estados Unidos
Texto completo
Añadir a Mi BVS
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XML
PubMed Links
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Nano Lett Año: 2022 Tipo del documento: Article Pais de publicación: Estados Unidos