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Electronic Metal-Support Interaction Modulation of Single-Atom Electrocatalysts for Rechargeable Zinc-Air Batteries.
Wu, Mingjie; Zhang, Gaixia; Wang, Weichao; Yang, Huaming; Rawach, Diane; Chen, Mengjun; Sun, Shuhui.
Afiliación
  • Wu M; Institut National de la Recherche Scientifique (INRS)-Centre Énergie Matériaux Télécommunications, Varennes, Québec, J3X 1P7, Canada.
  • Zhang G; Engineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan, 430074, China.
  • Wang W; Institut National de la Recherche Scientifique (INRS)-Centre Énergie Matériaux Télécommunications, Varennes, Québec, J3X 1P7, Canada.
  • Yang H; Department of Electronics, National Institute for Advanced Materials, Renewable Energy Conversion and Storage Center, Tianjin Key Laboratory of Photo-Electronic Thin Film Device and Technology, Nankai University, Tianjin, 300071, China.
  • Rawach D; Engineering Research Center of Nano-Geomaterials of Ministry of Education, China University of Geosciences, Wuhan, 430074, China.
  • Chen M; Department of Inorganic Materials, School of Minerals Processing and Bioengineering, Central South University, Changsha, 410083, China.
  • Sun S; Institut National de la Recherche Scientifique (INRS)-Centre Énergie Matériaux Télécommunications, Varennes, Québec, J3X 1P7, Canada.
Small Methods ; 6(3): e2100947, 2022 Mar.
Article en En | MEDLINE | ID: mdl-35037425
High-performance oxygen electrocatalysts play a key role in the widespread application of rechargeable Zn-air batteries (ZABs). Single-atom catalysts (SACs) with maximum atom efficiency and well-defined active sites have been recognized as promising alternatives of the present noble-metal-based catalysts for oxygen reduction reaction and oxygen evolution reaction. To improve their oxygen electrocatalysis activities and reveal the structure-activity relationship, many advanced synthesis and characterization methods have been developed to study the effects of 1) coordination and electronic structure of the metal centers and 2) morphology and stability of the conductive substrates. Herein, a detailed review of the recent advances of SACs with strong electronic metal-support interaction (EMSI) for rechargeable ZABs is provided. Great emphasis was placed on the EMSI forms and design strategies. Moreover, the importance and the impact of the atomic coordinating structure and the substrates on the oxygen electrocatalytic activity and stability are highlighted. Finally, future directions and perspectives on the development of SACs are also presented.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Methods Año: 2022 Tipo del documento: Article País de afiliación: Canadá Pais de publicación: Alemania
Texto completo
Añadir a Mi BVS
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Small Methods Año: 2022 Tipo del documento: Article País de afiliación: Canadá Pais de publicación: Alemania