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Novel Mitochondria-Targeting and Naphthalimide-based Fluorescent Probe for Detecting HClO in Living Cells.
Xu, Junhong; Wang, Chunyan; Ma, Qiujuan; Zhang, Hongtao; Tian, Meiju; Sun, Jingguo; Wang, Baiyan; Chen, Yacong.
Afiliación
  • Xu J; Department of Dynamical Engineering, North China University of Water Resources and Electric Power, Zhengzhou 450011, PR China.
  • Wang C; School of Pharmacy, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
  • Ma Q; School of Pharmacy, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
  • Zhang H; Department of Dynamical Engineering, North China University of Water Resources and Electric Power, Zhengzhou 450011, PR China.
  • Tian M; School of Pharmacy, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
  • Sun J; School of Pharmacy, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
  • Wang B; Key Discipline Laboratory of Basic Medicine, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
  • Chen Y; School of Pharmacy, Henan University of Traditional Chinese Medicine, Zhengzhou 450046, PR China.
ACS Omega ; 6(22): 14399-14409, 2021 Jun 08.
Article en En | MEDLINE | ID: mdl-34124462
As a key reactive oxygen species (ROS), hypochlorous acid (HClO) plays an important role in many physiological and pathological processes. The mitochondria-targeting probes for the highly sensitive detection of HClO are desirable. In present work, we designed and synthesized an original mitochondria-localizing and turn-on fluorescent probe for detecting HClO. 4-Aminonaphthalimide was employed as the fluorescent section, the (2-aminoethyl)-thiourea unit was utilized as a typical sensing unit, and the quaternized pyridinium moiety was used as a mitochondria-targeted localization group. When HClO was absent, the probe showed weak fluorescence. In the existence of HClO, the probe revealed a blue fluorescence. Moreover, the turn-on fluorescent probe was able to function in a broad pH scope. There was an excellent linearity between the fluorescence emission intensity at 488 nm and the concentrations of HClO in the range of 5.0 × 10-7 to 2.5 × 10-6 mol·L-1. Additionally, the probe had almost no cell toxicity and possessed an excellent mitochondria-localizing capability. Furthermore, the probe was able to image HClO in mitochondria of living PC-12 cells. The above remarkable properties illustrated that the probe was able to determine HClO in mitochondria of living cells.

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Omega Año: 2021 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Omega Año: 2021 Tipo del documento: Article Pais de publicación: Estados Unidos