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Kinetic selection of Pd4L2 metallocyclic and Pd6L3 trigonal prismatic assemblies.
O'Connor, Helen M; Coletta, Marco; Etcheverry-Berríos, Alvaro; Nichol, Gary S; Brechin, Euan K; Lusby, Paul J.
Afiliación
  • O'Connor HM; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
  • Coletta M; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
  • Etcheverry-Berríos A; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
  • Nichol GS; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
  • Brechin EK; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
  • Lusby PJ; EaStCHEM School of Chemistry, The University of Edinburgh, David Brewster Road, Edinburgh, EH9 3FJ, UK. E.Brechin@ed.ac.uk Paul.Lusby@ed.ac.uk.
Chem Commun (Camb) ; 56(79): 11799-11802, 2020 Oct 06.
Article en En | MEDLINE | ID: mdl-33021303
The self-assembly of Pd4L2 metallocylcic and Pd6L3 trigonal prismatic assemblies are described. The selection of one species over the other has been achieved by careful choice of ancilliary ligands, which switch the dynamics of the Pd-pyridine bonds such that a highly unusual and distorted smaller assembly can be kinetically trapped en route to the more energetically favourable larger species. Both assemblies provide promise as easy to access multicavity reaction vessels.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2020 Tipo del documento: Article Pais de publicación: Reino Unido
Texto completo
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XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Chem Commun (Camb) Asunto de la revista: QUIMICA Año: 2020 Tipo del documento: Article Pais de publicación: Reino Unido