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Atomic force microscopy imaging of delignified secondary cell walls in liquid conditions facilitates interpretation of wood ultrastructure.
Adobes-Vidal, Maria; Frey, Marion; Keplinger, Tobias.
Afiliación
  • Adobes-Vidal M; Wood Materials Science, ETH Zürich, Stefano-Franscini-Platz 3, 8093 Zürich, Switzerland; Laboratory for Cellulose & Wood Materials, Empa, Überlandstrasse 129, 8600 Dübendorf, Switzerland. Electronic address: mariaad@ethz.ch.
  • Frey M; Wood Materials Science, ETH Zürich, Stefano-Franscini-Platz 3, 8093 Zürich, Switzerland; Laboratory for Cellulose & Wood Materials, Empa, Überlandstrasse 129, 8600 Dübendorf, Switzerland.
  • Keplinger T; Wood Materials Science, ETH Zürich, Stefano-Franscini-Platz 3, 8093 Zürich, Switzerland; Laboratory for Cellulose & Wood Materials, Empa, Überlandstrasse 129, 8600 Dübendorf, Switzerland. Electronic address: tkeplinger@ethz.ch.
J Struct Biol ; 211(2): 107532, 2020 08 01.
Article en En | MEDLINE | ID: mdl-32442716
Deep understanding of the physicochemical and structural characteristics of wood at the nanoscale is essential for improving wood usage in biorefining and advancing new high performance materials design. Herein, we use in situ atomic force microscopy and a simple delignification treatment to elucidate the nanoscale architecture of individual secondary cell wall layers. Advantages of this approach are: (i) minimal sample preparation that reduces the introduction of potential artifacts; (ii) prevention of structural rearrangements due to dehydration; (iii) increased accessibility to structural details masked by the lignin matrix; and (iv) possibility to complement results with other analytical techniques without sample manipulation. The methodology permits the visualization of parallel and helicoidally arranged microfibril aggregates in the S1 layer and the determination of lignin contribution to microfibril aggregates forming S2 layers. Cellulose and hemicelluloses constitute the core of the aggregates with a mean diameter of approximately 19 nm, and lignin encloses the core forming single structural entities of about 30 nm diameter. Furthermore, we highlight the implications of sample preparation and imaging parameters on the characterization of microfibril aggregates by AFM.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Madera / Pared Celular / Lignina Idioma: En Revista: J Struct Biol Asunto de la revista: BIOLOGIA MOLECULAR Año: 2020 Tipo del documento: Article Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Madera / Pared Celular / Lignina Idioma: En Revista: J Struct Biol Asunto de la revista: BIOLOGIA MOLECULAR Año: 2020 Tipo del documento: Article Pais de publicación: Estados Unidos