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Mitochondria-targeted triphenylphosphonium-based compounds do not affect estrogen receptor α.
Zinovkina, Ludmila A; Galivondzhyan, Alina K; Prikhodko, Anastasia S; Galkin, Ivan I; Zinovkin, Roman A.
Afiliación
  • Zinovkina LA; Faculty of Bioengineering and Bioinformatics, Lomonosov Moscow State University, Moscow, Russia.
  • Galivondzhyan AK; Institute of Mitoengineering, Moscow State University, Moscow, Russia.
  • Prikhodko AS; Faculty of Bioengineering and Bioinformatics, Lomonosov Moscow State University, Moscow, Russia.
  • Galkin II; Institute of Mitoengineering, Moscow State University, Moscow, Russia.
  • Zinovkin RA; Belozersky Institute of Physico-Chemical Biology, Lomonosov Moscow State University, Moscow, Russia.
PeerJ ; 8: e8803, 2020.
Article en En | MEDLINE | ID: mdl-32257641
BACKGROUND: Targeting negatively charged mitochondria is often achieved using triphenylphosphonium (TPP) cations. These cationic vehicles may possess biological activity, and a docking study indicates that TPP-moieties may act as modulators of signaling through the estrogen receptor α (ERα). Moreover, in vivo and in vitro experiments revealed the estrogen-like effects of TPP-based compounds. Here, we tested the hypothesis that TPP-based compounds regulate the activity of ERα. METHODS: We used ERa-positive and ERα-negative human breast adenocarcinoma cell lines (MCF-7 and MDA-MB-231, respectively). Cell proliferation was measured using a resazurin cell growth assay and a real-time cell analyzer assay. Cell cycle progression was analyzed using flow cytometry. Real-time PCR was used to assess mRNA expression of endogenous estrogen-responsive genes. Luciferase activity was measured to evaluate transcription driven by estrogen-responsive promoters in cells transfected with an estrogen response element (ERE)3-luciferase expression vector. RESULTS: The TPP-based molecules SkQ1 and C12TPP, as well as the rhodamine-based SkQR1, did not increase the proliferation or alter the cell cycle progression of MCF-7 cells. In contrast, 17ß estradiol increased the proliferation of MCF-7 cells and the proportion of cells in the S/G2/M-phases of the cell cycle. TPP-based compounds did not affect the induction of transcription of an ERE-luciferase expression vector in vitro, and SkQ1 did not alter the levels of expression of estrogen-dependent genes encoding GREB1, TFF1, COX6, and IGFBP4. CONCLUSION: TPP-based compounds do not possess properties typical of ERα agonists.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: PeerJ Año: 2020 Tipo del documento: Article País de afiliación: Rusia Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: PeerJ Año: 2020 Tipo del documento: Article País de afiliación: Rusia Pais de publicación: Estados Unidos