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Hierarchical Mesoporous MXene-NiCoP Electrocatalyst for Water-Splitting.
Yue, Qin; Sun, Jiao; Chen, Shan; Zhou, Yu; Li, Hongjian; Chen, Yang; Zhang, Ruya; Wei, Guangfeng; Kang, Yijin.
Afiliación
  • Yue Q; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Sun J; Shanghai Key Laboratory of Chemical Assessment and Sustainability, School of Chemical Science and Engineering, Tongji University, Shanghai 200092, China.
  • Chen S; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Zhou Y; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Li H; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Chen Y; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Zhang R; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
  • Wei G; Shanghai Key Laboratory of Chemical Assessment and Sustainability, School of Chemical Science and Engineering, Tongji University, Shanghai 200092, China.
  • Kang Y; Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China.
ACS Appl Mater Interfaces ; 12(16): 18570-18577, 2020 Apr 22.
Article en En | MEDLINE | ID: mdl-32237730
The utilization of nonprecious metal electrocatalysts for water-splitting may be the ultimate solution for sustainable and clean hydrogen energy. MXene, an emerging two-dimensional material, exhibits many unique properties such as possible metal-like conductivity, hydrophilic surface, and rich chemistry, rendering a group of promising catalysts and catalyst support materials. In this study, exfoliated Ti3C2 MXenes serve as a substrate to perpendicularly grow uniform mesoporous NiCoP nanosheets through an in situ interface-growth strategy and subsequent phosphorization. The obtained Ti3C2@mNiCoP materials with a stable hierarchical sandwich structure possess excellent conductivity, large surface area, and uniform mesopores with high pore volume. With these beneficial properties, the Ti3C2@mNiCoP material exhibits superior overall water-splitting performance compared with that of its building-block counterparts, matching the state-of-the-art water-splitting electrocatalysts.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2020 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos
Texto completo
Añadir a Mi BVS
Imprimir
XML
PubMed Links
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: ACS Appl Mater Interfaces Asunto de la revista: BIOTECNOLOGIA / ENGENHARIA BIOMEDICA Año: 2020 Tipo del documento: Article País de afiliación: China Pais de publicación: Estados Unidos