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Efficient tandem solar cells with solution-processed perovskite on textured crystalline silicon.
Hou, Yi; Aydin, Erkan; De Bastiani, Michele; Xiao, Chuanxiao; Isikgor, Furkan H; Xue, Ding-Jiang; Chen, Bin; Chen, Hao; Bahrami, Behzad; Chowdhury, Ashraful H; Johnston, Andrew; Baek, Se-Woong; Huang, Ziru; Wei, Mingyang; Dong, Yitong; Troughton, Joel; Jalmood, Rawan; Mirabelli, Alessandro J; Allen, Thomas G; Van Kerschaver, Emmanuel; Saidaminov, Makhsud I; Baran, Derya; Qiao, Qiquan; Zhu, Kai; De Wolf, Stefaan; Sargent, Edward H.
Afiliación
  • Hou Y; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Aydin E; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • De Bastiani M; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Xiao C; National Renewable Energy Laboratory (NREL), Golden, CO 80401, USA.
  • Isikgor FH; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Xue DJ; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Chen B; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Chen H; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Bahrami B; Department of Electrical Engineering, Center for Advanced Photovoltaics, South Dakota State University, Brookings, SD 57007, USA.
  • Chowdhury AH; Department of Electrical Engineering, Center for Advanced Photovoltaics, South Dakota State University, Brookings, SD 57007, USA.
  • Johnston A; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Baek SW; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Huang Z; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Wei M; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Dong Y; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Troughton J; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Jalmood R; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Mirabelli AJ; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Allen TG; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Van Kerschaver E; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Saidaminov MI; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada.
  • Baran D; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia.
  • Qiao Q; Department of Electrical Engineering, Center for Advanced Photovoltaics, South Dakota State University, Brookings, SD 57007, USA.
  • Zhu K; National Renewable Energy Laboratory (NREL), Golden, CO 80401, USA.
  • De Wolf S; KAUST Solar Center (KSC), Physical Sciences and Engineering Division (PSE), King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Kingdom of Saudi Arabia. stefaan.dewolf@kaust.edu.sa ted.sargent@utoronto.ca.
  • Sargent EH; Department of Electrical and Computer Engineering, University of Toronto, Toronto, Ontario M5S 1A4, Canada. stefaan.dewolf@kaust.edu.sa ted.sargent@utoronto.ca.
Science ; 367(6482): 1135-1140, 2020 03 06.
Article en En | MEDLINE | ID: mdl-32139544
Stacking solar cells with decreasing band gaps to form tandems presents the possibility of overcoming the single-junction Shockley-Queisser limit in photovoltaics. The rapid development of solution-processed perovskites has brought perovskite single-junction efficiencies >20%. However, this process has yet to enable monolithic integration with industry-relevant textured crystalline silicon solar cells. We report tandems that combine solution-processed micrometer-thick perovskite top cells with fully textured silicon heterojunction bottom cells. To overcome the charge-collection challenges in micrometer-thick perovskites, we enhanced threefold the depletion width at the bases of silicon pyramids. Moreover, by anchoring a self-limiting passivant (1-butanethiol) on the perovskite surfaces, we enhanced the diffusion length and further suppressed phase segregation. These combined enhancements enabled an independently certified power conversion efficiency of 25.7% for perovskite-silicon tandem solar cells. These devices exhibited negligible performance loss after a 400-hour thermal stability test at 85°C and also after 400 hours under maximum power point tracking at 40°C.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Science Año: 2020 Tipo del documento: Article País de afiliación: Canadá Pais de publicación: Estados Unidos
Texto completo
Añadir a Mi BVS
Imprimir
XML
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Science Año: 2020 Tipo del documento: Article País de afiliación: Canadá Pais de publicación: Estados Unidos