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A frontal analysis combined with a simultaneous chromatographic analysis of macromolecules using a single chromatographic system.
Ambrozic, Rok; Modic, Petra; Hribar, Gorazd; Podgornik, Ales.
Afiliación
  • Ambrozic R; Faculty for Chemistry and Chemical Technology, University of Ljubljana, Vecna pot 113, 1000 Ljubljana, Slovenia.
  • Modic P; Faculty for Chemistry and Chemical Technology, University of Ljubljana, Vecna pot 113, 1000 Ljubljana, Slovenia.
  • Hribar G; Lek d. d., Verovskova 57, 1526 Ljubljana, Slovenia.
  • Podgornik A; Faculty for Chemistry and Chemical Technology, University of Ljubljana, Vecna pot 113, 1000 Ljubljana, Slovenia; COBIK, Tovarniska 26, 5270 Ajdovscina, Slovenia. Electronic address: ales.podgornik@fkkt.uni-lj.si.
J Chromatogr A ; 1610: 460571, 2020 Jan 11.
Article en En | MEDLINE | ID: mdl-31708219
A chromatographic system was adapted to allow monitoring of eluent of preparative column via absorbance and with the chromatographic analysis of the target macromolecule on the same chromatographic system. The proposed approach was tested on important macromolecules, such as monoclonal antibodies, monoclonal antibody aggregates and plasmid DNA (pDNA). A frontal analysis was made on the preparative column, while a chromatographic on-line analysis was performed by sequentially injecting the preparative column outlet on a convection-based analytical column, operating on the same chromatographic system. Cation and/or anion exchangers were used as the chromatographic media (along with a protein A), depending on the sample to be purified. The method was found to be robust and reproducible. To adjust the limit of detection, an algorithm varying the number of injections was used, enabling accurate monitoring of an early breakthrough for concentrations below 1% of the feed concentration. The accuracy varies according to the applied flow rate, but it is typically in the range of few percent, or even below. Due to its simplicity and flexibility, the proposed method can be easily adapted to a pharmaceutical environment.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Cromatografía por Intercambio Iónico Idioma: En Revista: J Chromatogr A Año: 2020 Tipo del documento: Article País de afiliación: Eslovenia Pais de publicación: Países Bajos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Cromatografía por Intercambio Iónico Idioma: En Revista: J Chromatogr A Año: 2020 Tipo del documento: Article País de afiliación: Eslovenia Pais de publicación: Países Bajos