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Improving Mechanical Properties for Extrusion-Based Additive Manufacturing of Poly(Lactic Acid) by Annealing and Blending with Poly(3-Hydroxybutyrate).
Wang, Sisi; Daelemans, Lode; Fiorio, Rudinei; Gou, Maling; D'hooge, Dagmar R; De Clerck, Karen; Cardon, Ludwig.
Afiliación
  • Wang S; Centre for Polymer and Material Technologies (CPMT), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Sisi.Wang@ugent.be.
  • Daelemans L; Centre for Textiles Science and Engineering (CTSE), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Lode.Daelemans@UGent.be.
  • Fiorio R; Centre for Polymer and Material Technologies (CPMT), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Rudinei.Fiorio@UGent.be.
  • Gou M; State Key Laboratory of Biotherapy and Cancer Center, West China Hospital, Sichuan University, Chengdu 610041, China. goumaling@scu.edu.cn.
  • D'hooge DR; Centre for Textiles Science and Engineering (CTSE), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Dagmar.Dhooge@UGent.be.
  • De Clerck K; Laboratory for Chemical Technology (LCT), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Dagmar.Dhooge@UGent.be.
  • Cardon L; Centre for Textiles Science and Engineering (CTSE), Department of Materials, Textiles and Chemical Engineering, Ghent University, 9052 Zwijnaarde, Belgium. Karen.DeClerck@UGent.be.
Polymers (Basel) ; 11(9)2019 Sep 19.
Article en En | MEDLINE | ID: mdl-31546970
Based on differential scanning calorimetry (DSC), X-ray diffraction (XRD) analysis, polarizing microscope (POM), and scanning electron microscopy (SEM) analysis, strategies to close the gap on applying conventional processing optimizations for the field of 3D printing and to specifically increase the mechanical performance of extrusion-based additive manufacturing of poly(lactic acid) (PLA) filaments by annealing and/or blending with poly(3-hydroxybutyrate) (PHB) were reported. For filament printing at 210 °C, the PLA crystallinity increased significantly upon annealing. Specifically, for 2 h of annealing at 100 °C, the fracture surface became sufficiently coarse such that the PLA notched impact strength increased significantly (15 kJ m-2). The Vicat softening temperature (VST) increased to 160 °C, starting from an annealing time of 0.5 h. Similar increases in VST were obtained by blending with PHB (20 wt.%) at a lower printing temperature of 190 °C due to crystallization control. For the blend, the strain at break increased due to the presence of a second phase, with annealing only relevant for enhancing the modulus.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Polymers (Basel) Año: 2019 Tipo del documento: Article País de afiliación: Bélgica Pais de publicación: Suiza

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Polymers (Basel) Año: 2019 Tipo del documento: Article País de afiliación: Bélgica Pais de publicación: Suiza