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Reaction of Electrons with DNA: Radiation Damage to Radiosensitization.
Kumar, Anil; Becker, David; Adhikary, Amitava; Sevilla, Michael D.
Afiliación
  • Kumar A; Department of Chemistry, Oakland University, Rochester, MI 48309, USA.
  • Becker D; Department of Chemistry, Oakland University, Rochester, MI 48309, USA.
  • Adhikary A; Department of Chemistry, Oakland University, Rochester, MI 48309, USA.
  • Sevilla MD; Department of Chemistry, Oakland University, Rochester, MI 48309, USA. sevilla@oakland.edu.
Int J Mol Sci ; 20(16)2019 Aug 16.
Article en En | MEDLINE | ID: mdl-31426385
This review article provides a concise overview of electron involvement in DNA radiation damage. The review begins with the various states of radiation-produced electrons: Secondary electrons (SE), low energy electrons (LEE), electrons at near zero kinetic energy in water (quasi-free electrons, (e-qf)) electrons in the process of solvation in water (presolvated electrons, e-pre), and fully solvated electrons (e-aq). A current summary of the structure of e-aq, and its reactions with DNA-model systems is presented. Theoretical works on reduction potentials of DNA-bases were found to be in agreement with experiments. This review points out the proposed role of LEE-induced frank DNA-strand breaks in ion-beam irradiated DNA. The final section presents radiation-produced electron-mediated site-specific formation of oxidative neutral aminyl radicals from azidonucleosides and the evidence of radiosensitization provided by these aminyl radicals in azidonucleoside-incorporated breast cancer cells.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Daño del ADN / ADN / Electrones Límite: Animals / Humans Idioma: En Revista: Int J Mol Sci Año: 2019 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Suiza

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Daño del ADN / ADN / Electrones Límite: Animals / Humans Idioma: En Revista: Int J Mol Sci Año: 2019 Tipo del documento: Article País de afiliación: Estados Unidos Pais de publicación: Suiza