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Anti-inflammatory and diuretic effects of the diterpene ent-dihydrotucumanoic acid.
Alonso-Castro, Angel Josabad; Arana-Argáez, Víctor E; Deveze-Alvarez, Martha Alicia; Chan-Zapata, Ivan; Torres-Romero, Julio Cesar; Carranza-Álvarez, Candy; Luna-Rubio, Sarahí; González-Chávez, Marco M; Zapata-Morales, Juan R; Aragón-Martínez, Othoniel H; Ramírez-Morales, Marco Antonio.
Afiliación
  • Alonso-Castro AJ; Departamento de Farmacia, División de Ciencias Naturales y Exactas, Universidad de Guanajuato, Guanajuato, Guanajuato, Mexico.
  • Arana-Argáez VE; Facultad de Química, Universidad Autónoma de Yucatán, Mérida, Yucatán, Mexico.
  • Deveze-Alvarez MA; Departamento de Farmacia, División de Ciencias Naturales y Exactas, Universidad de Guanajuato, Guanajuato, Guanajuato, Mexico.
  • Chan-Zapata I; Facultad de Química, Universidad Autónoma de Yucatán, Mérida, Yucatán, Mexico.
  • Torres-Romero JC; Facultad de Química, Universidad Autónoma de Yucatán, Mérida, Yucatán, Mexico.
  • Carranza-Álvarez C; Unidad Académica Multidisciplinaria zona Huasteca, Universidad Autónoma de San Luis Potosí, Ciudad Valles, San Luis Potosí, Mexico.
  • Luna-Rubio S; Unidad Académica Multidisciplinaria zona Huasteca, Universidad Autónoma de San Luis Potosí, Ciudad Valles, San Luis Potosí, Mexico.
  • González-Chávez MM; Facultad de Ciencias Químicas, Universidad Autónoma de San Luis Potosí, San Luis Potosí, San Luis Potosí, Mexico.
  • Zapata-Morales JR; Departamento de Farmacia, División de Ciencias Naturales y Exactas, Universidad de Guanajuato, Guanajuato, Guanajuato, Mexico.
  • Aragón-Martínez OH; Facultad de Medicina, Universidad Autónoma de San Luis Potosí, San Luis Potosí, San Luis Potosí, Mexico.
  • Ramírez-Morales MA; Departamento de Farmacia, División de Ciencias Naturales y Exactas, Universidad de Guanajuato, Guanajuato, Guanajuato, Mexico.
Drug Dev Res ; 80(6): 800-806, 2019 09.
Article en En | MEDLINE | ID: mdl-31243798
Gymnosperma glutinosum (Spreng) Less (Asteraceae) is a shrub used in traditional medicine for the treatment of inflammatory and renal diseases. The ent-dihydrotucumanoic acid (DTA) is a diterpene obtained from G. glutinosum. This study evaluated the antioxidant, genotoxic, and diuretic properties of DTA, as well as its in vitro and in vivo anti-inflammatory actions. The antioxidant actions of DTA were assessed with the 2,2'-azino-bis (3-ethylbenzothiazoline-6-sulphonic acid) (ABTS), ferric reducing antioxidant power (FRAP), and 2,2'-diphenyl-1-picrylhydrazyl (DPPH) assays, the genotoxic action was assessed with the comet assay, and the diuretic effects of DTA were assessed using metabolic cages. The anti-inflammatory actions were evaluated using primary murine peritoneal macrophages stimulated with LPS and the λ-carrageenan-induced hind paw edema test. DTA lacked antioxidant (IC50 > 25,000 µg/mL) activity in the ABTS, FRAP, and DPPH assays. DTA at 500-1,000 µg/mL showed moderate genotoxicity. In LPS-stimulated macrophages, DTA showed IC50 values of 74.85 µg/mL (TNF-α) and 58.12 µg/mL (NO), whereas the maximum inhibition of IL-6 (24%) and IL-1ß (36%) was recorded at 200 µg/mL. DTA induced in vivo anti-inflammatory effects with ED50 = 124.3 mg/kg. The in vitro anti-inflammatory activity of DTA seems to be associated with the decrease in the release of TNF-α and NO. DTA promoted the excretion of urine (ED50 = 86.9 mg/kg), Na+ (ED50 = 66.7 mg/kg), and K+ (ED50 = 8.6 mg/kg). The coadministration of DTA with L-NAME decreased the urinary excretion shown by DTA alone. Therefore, the diuretic activity is probably associated with the participation of nitric oxide synthase. In conclusion, DTA exerted anti-inflammatory and diuretic effects, but lacked antioxidant effects.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Diterpenos / Diuréticos / Antiinflamatorios / Antioxidantes Idioma: En Revista: Drug Dev Res Año: 2019 Tipo del documento: Article País de afiliación: México Pais de publicación: Estados Unidos

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Diterpenos / Diuréticos / Antiinflamatorios / Antioxidantes Idioma: En Revista: Drug Dev Res Año: 2019 Tipo del documento: Article País de afiliación: México Pais de publicación: Estados Unidos