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Structural Flexibility in Activated Carbon Materials Prepared under Harsh Activation Conditions.
Gomes Ferreira de Paula, Fabiano; Campello-Gómez, Ignacio; Ortega, Paulo Fernando Ribeiro; Rodríguez-Reinoso, Francisco; Martínez-Escandell, Manuel; Silvestre-Albero, Joaquín.
Afiliación
  • Gomes Ferreira de Paula F; Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica-IUMA, Universidad de Alicante, Ctra. San Vicente-Alicante s/n, E-03690 San Vicente del Raspeig, Spain. fabianogfp@gmail.com.
  • Campello-Gómez I; Universidade Federal de Minas Gerais (UFMG), Av. Antônio Carlos 6627, Belo Horizonte, Minas Gerais 31270-901, Brazil. fabianogfp@gmail.com.
  • Ortega PFR; Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica-IUMA, Universidad de Alicante, Ctra. San Vicente-Alicante s/n, E-03690 San Vicente del Raspeig, Spain. nachocampeg@gmail.com.
  • Rodríguez-Reinoso F; Departamento de Química, Centro Federal de Educaçao Tecnológica de Minas Gerais, Av. Amazonas 5253, Nova Suíça, Belo Horizonte 30421-169, Brazil. pauloortega@cefetmg.br.
  • Martínez-Escandell M; Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica-IUMA, Universidad de Alicante, Ctra. San Vicente-Alicante s/n, E-03690 San Vicente del Raspeig, Spain. reinoso@ua.es.
  • Silvestre-Albero J; Laboratorio de Materiales Avanzados, Departamento de Química Inorgánica-IUMA, Universidad de Alicante, Ctra. San Vicente-Alicante s/n, E-03690 San Vicente del Raspeig, Spain. manolo.m@ua.es.
Materials (Basel) ; 12(12)2019 Jun 20.
Article en En | MEDLINE | ID: mdl-31226832
Although traditionally high-surface area carbon materials have been considered as rigid structures with a disordered three dimensional (3D) network of graphite microdomains associated with a limited electrical conductivity (highly depending on the porous structure and surface chemistry), here we show for the first time that this is not the case for activated carbon materials prepared using harsh activation conditions (e.g., KOH activation). In these specific samples a clear structural re-orientation can be observed upon adsorption of different organic molecules, the structural changes giving rise to important changes in the electrical resistivity of the material. Whereas short chain hydrocarbons and their derivatives give rise to an increased resistivity, the contrary occurs for longer-chain hydrocarbons and/or alcohols. The high sensitivity of these high-surface area carbon materials towards these organic molecules opens the gate towards their application for sensing devices.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Materials (Basel) Año: 2019 Tipo del documento: Article País de afiliación: España Pais de publicación: Suiza

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Idioma: En Revista: Materials (Basel) Año: 2019 Tipo del documento: Article País de afiliación: España Pais de publicación: Suiza