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Gel electrophoresis in combination with laser ablation-inductively coupled plasma mass spectrometry to quantify the interaction of cisplatin with human serum albumin.
Sullivan, Matthew P; Morrow, Stuart J; Goldstone, David C; Hartinger, Christian G.
Afiliación
  • Sullivan MP; School of Chemical Sciences, University of Auckland, Auckland, New Zealand.
  • Morrow SJ; School of Biological Sciences, University of Auckland, Auckland, New Zealand.
  • Goldstone DC; School of Chemical Sciences, University of Auckland, Auckland, New Zealand.
  • Hartinger CG; School of Biological Sciences, University of Auckland, Auckland, New Zealand.
Electrophoresis ; 40(18-19): 2329-2335, 2019 09.
Article en En | MEDLINE | ID: mdl-31087392
Cisplatin and its second and third generation analogues are widely used in the treatment of cancer. To study their reactions with proteins, we present a method based on SDS-PAGE separation and laser ablation-inductively coupled plasma-mass spectrometry (LA-ICP-MS) for platinum detection in the reaction between human serum albumin (HSA) and cisplatin. We developed matrix-matched standards of HSA/cisplatin mixtures and used them to quantify the amount of adducts formed at different HSA:cisplatin ratios. We noted that cisplatin incubation with HSA resulted in the formation of higher order HSA n-mers, depending on the amount of cisplatin added. This caused a depletion of the HSA dimer bands, while the majority of HSA was present as the monomer. Inducing the formation of such higher molecular weight species may have an impact on the mode of action of metallodrugs.
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Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Espectrometría de Masas / Cisplatino / Albúmina Sérica Humana Tipo de estudio: Guideline Límite: Humans Idioma: En Revista: Electrophoresis Año: 2019 Tipo del documento: Article País de afiliación: Nueva Zelanda Pais de publicación: Alemania

Texto completo: 1 Colección: 01-internacional Base de datos: MEDLINE Asunto principal: Espectrometría de Masas / Cisplatino / Albúmina Sérica Humana Tipo de estudio: Guideline Límite: Humans Idioma: En Revista: Electrophoresis Año: 2019 Tipo del documento: Article País de afiliación: Nueva Zelanda Pais de publicación: Alemania